PMID- 17966860
OWN - NLM
STAT- MEDLINE
DCOM- 20080124
LR  - 20190911
IS  - 1001-0742 (Print)
IS  - 1001-0742 (Linking)
VI  - 19
IP  - 8
DP  - 2007
TI  - Degradation of 2,4-dichlorophenol with a novel TiO2/Ti-Fe-graphite felt 
      photoelectrocatalytic oxidation process.
PG  - 1020-4
AB  - Degradation of 2,4-dichlorophenol (2,4-DCP) was studied in a novel 
      three-electrode photoelectrocatalytic (PEC) integrative oxidation process, and 
      the factors influencing the degradation rate, such as applied current, flow speed 
      of O2, pH, adscititious voltage and initial 2,4-DCP concentration were 
      investigated and optimized. H2O2 was produced nearby cathode and Fe2+ 
      continuously generated from Fe anode in solution when current and O2 were 
      applied, so, main reactions, H2O2-assisted TiO2 PEC oxidation and E-Fenton 
      reaction, occurred during degradation of 2,4-DCP in this integrative system. The 
      degradation ratio of 2,4-DCP was 93% in this integrative oxidation process, while 
      it was only 31% in E-Fenton process and 46% in H2O2-assisted TiO2 PEC process. 
      So, it revealed that the degradation of 2,4-DCP was improved greatly by 
      photoelectrical cooperation effect. By the investigation of pH, it showed that 
      this integrative process could work well in a wide pH range from pH 3 to pH 9.
FAU - Zhao, Bao-xiu
AU  - Zhao BX
AD  - School of Municipal and Environmental Engineering, Harbin Institute of 
      Technology, Harbin 150090, China. zhaobaoxiuhit@163.com
FAU - Li, Xiang-zhong
AU  - Li XZ
FAU - Wang, Peng
AU  - Wang P
LA  - eng
PT  - Journal Article
PT  - Research Support, Non-U.S. Gov't
PL  - Netherlands
TA  - J Environ Sci (China)
JT  - Journal of environmental sciences (China)
JID - 100967627
RN  - 0 (Chlorophenols)
RN  - 0 (Water Pollutants, Chemical)
RN  - 15FIX9V2JP (titanium dioxide)
RN  - 7782-42-5 (Graphite)
RN  - BBX060AN9V (Hydrogen Peroxide)
RN  - D1JT611TNE (Titanium)
RN  - E1UOL152H7 (Iron)
RN  - R669TG1950 (2,4-dichlorophenol)
RN  - S88TT14065 (Oxygen)
SB  - IM
MH  - Catalysis
MH  - Chlorophenols/*chemistry/*radiation effects
MH  - Electrochemistry
MH  - Graphite/*chemistry
MH  - Hydrogen Peroxide/chemistry
MH  - Hydrogen-Ion Concentration
MH  - Iron/*chemistry
MH  - Oxidation-Reduction
MH  - Oxygen/chemistry
MH  - Photochemistry
MH  - Titanium/*chemistry
MH  - *Ultraviolet Rays
MH  - Water Pollutants, Chemical/chemistry/radiation effects
MH  - Water Purification/methods
EDAT- 2007/10/31 09:00
MHDA- 2008/01/25 09:00
CRDT- 2007/10/31 09:00
PHST- 2007/10/31 09:00 [pubmed]
PHST- 2008/01/25 09:00 [medline]
PHST- 2007/10/31 09:00 [entrez]
AID - 10.1016/s1001-0742(07)60165-x [doi]
PST - ppublish
SO  - J Environ Sci (China). 2007;19(8):1020-4. doi: 10.1016/s1001-0742(07)60165-x.