PMID- 23452228 OWN - NLM STAT- MEDLINE DCOM- 20140325 LR - 20181202 IS - 1520-5851 (Electronic) IS - 0013-936X (Linking) VI - 47 IP - 7 DP - 2013 Apr 2 TI - Monsoon-driven transport of organochlorine pesticides and polychlorinated biphenyls to the Tibetan Plateau: three year atmospheric monitoring study. PG - 3199-208 LID - 10.1021/es305201s [doi] AB - Due to the influence of the Indian monsoon system, air mass transport in and to the Tibetan Plateau shows obvious seasonality. In order to assess the responses of atmospheric concentrations of persistent organic pollutants (POPs) to the Indian Monsoon fluctuation patterns, a three year air monitoring program (2008-2011) was conducted in an observation station close to the Yarlung Tsangpo Grand Canyon, southeastern Tibetan Plateau. The air concentrations of polychlorinated biphenyls (PCBs) and hexachlorocyclohexanes (HCHs) are generally comparable to those of other remote regions, whereas the concentrations of DDTs are much higher than reported for the polar regions, the North American Rocky Mountains, and the European Alps. The concentrations of DDTs and PCBs were strongly linked to the cyclic patterns of the Indian monsoon, displaying higher values in the monsoon season (May-September) and lower values in the nonmonsoon season (November-March). A "bimodal" pattern was observed for alpha- and gamma-HCH, with higher concentrations in spring and autumn and lower concentrations in the summer (monsoon season). Rain scavenging in the monsoon season likely resulted in the lower HCH concentrations in the atmosphere. This paper sheds lights on the role the Indian monsoon plays on the atmospheric transport of POPs to the Tibetan Plateau. FAU - Sheng, Jiujiang AU - Sheng J AD - Key Laboratory of Tibetan Environment Changes and Land Surface Processes, Institute of Tibetan Plateau Research, Chinese Academy of Sciences, Beijing 100101, China. FAU - Wang, Xiaoping AU - Wang X FAU - Gong, Ping AU - Gong P FAU - Joswiak, Daniel R AU - Joswiak DR FAU - Tian, Lide AU - Tian L FAU - Yao, Tandong AU - Yao T FAU - Jones, Kevin C AU - Jones KC LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20130311 PL - United States TA - Environ Sci Technol JT - Environmental science & technology JID - 0213155 RN - 0 (Air Pollutants) RN - 0 (Hydrocarbons, Chlorinated) RN - 0 (Pesticides) RN - 59NEE7PCAB (Hexachlorocyclohexane) RN - CIW5S16655 (DDT) RN - DFC2HB4I0K (Polychlorinated Biphenyls) SB - IM MH - Air Pollutants/analysis MH - Atmosphere/*chemistry MH - DDT/analysis MH - Environmental Monitoring/*methods MH - Geography MH - Hexachlorocyclohexane/analysis MH - Hydrocarbons, Chlorinated/*analysis MH - India MH - Models, Chemical MH - Pesticides/*analysis MH - Polychlorinated Biphenyls/*analysis MH - *Seasons MH - Tibet MH - *Transportation MH - Volatilization EDAT- 2013/03/05 06:00 MHDA- 2014/03/26 06:00 CRDT- 2013/03/05 06:00 PHST- 2013/03/05 06:00 [entrez] PHST- 2013/03/05 06:00 [pubmed] PHST- 2014/03/26 06:00 [medline] AID - 10.1021/es305201s [doi] PST - ppublish SO - Environ Sci Technol. 2013 Apr 2;47(7):3199-208. doi: 10.1021/es305201s. Epub 2013 Mar 11.