PMID- 23933454 OWN - NLM STAT- MEDLINE DCOM- 20140630 LR - 20131112 IS - 1879-1026 (Electronic) IS - 0048-9697 (Linking) VI - 466-467 DP - 2014 Jan 1 TI - Polybrominated diphenyl ethers in farmland soils: source characterization, deposition contribution and apportionment. PG - 524-32 LID - S0048-9697(13)00839-5 [pii] LID - 10.1016/j.scitotenv.2013.07.058 [doi] AB - Polybrominated diphenyl ethers (PBDEs), a group of persistent organic pollutants (POPs), are caused for concern recently due to their adverse health effects and environmental ubiquity. In this study, atmospheric and soil PBDE levels in Taizhou, one of the largest WEEE dismantling areas in the world, were measured, ranging from 884 to 2791 pg m(-3) with an average of 1968 pg m(-3) for atmosphere and 2.96 to 200 ng g(-1)dry weight (dw) with the mean of 65.2 ng g(-1)dw for farmland soils, respectively. The close connection between soil PBDE accumulation and atmospheric deposition was also revealed by the estimation of the annual PBDE deposition flux (3.1 +/- 0.9 mg m(-2)a(-1)) and the similarity between deposited congener pattern and soil congener profile. Positive matrix factorization (PMF) was conducted to extract possible sources of farmland soil PBDEs and to calculate their contributions. Based on the measured source profiles of PBDE-related activities, five sources were identified representing WEEE dumping, WEEE dismantling, WEEE open burning, residential waste dismantling, and residential waste open burning. WEEE-related recycling activities contributed primary percentage (52%) to farmland soil PBDE concentration, and open burning was an important pathway for PBDEs entering the environment. CI - (c) 2013. FAU - Dong, Yian AU - Dong Y AD - State Key Joint Laboratory for Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China. FAU - Li, Li AU - Li L FAU - Bie, Pengju AU - Bie P FAU - Jia, Shenglan AU - Jia S FAU - Wang, Qiang AU - Wang Q FAU - Huang, Zhi AU - Huang Z FAU - Qiu, Xinghua AU - Qiu X FAU - Zhang, Jianbo AU - Zhang J FAU - Hu, Jianxin AU - Hu J LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20130810 PL - Netherlands TA - Sci Total Environ JT - The Science of the total environment JID - 0330500 RN - 0 (Air Pollutants) RN - 0 (Halogenated Diphenyl Ethers) RN - 0 (Soil Pollutants) SB - IM MH - Agriculture MH - Air Pollutants/*analysis MH - China MH - Electronic Waste/*analysis MH - Environmental Monitoring MH - Gas Chromatography-Mass Spectrometry MH - Halogenated Diphenyl Ethers/*analysis MH - Soil Pollutants/*analysis OTO - NOTNLM OT - Atmospheric deposition OT - Farmland soil OT - PBDEs OT - PMF EDAT- 2013/08/13 06:00 MHDA- 2014/07/01 06:00 CRDT- 2013/08/13 06:00 PHST- 2013/03/17 00:00 [received] PHST- 2013/07/08 00:00 [revised] PHST- 2013/07/16 00:00 [accepted] PHST- 2013/08/13 06:00 [entrez] PHST- 2013/08/13 06:00 [pubmed] PHST- 2014/07/01 06:00 [medline] AID - S0048-9697(13)00839-5 [pii] AID - 10.1016/j.scitotenv.2013.07.058 [doi] PST - ppublish SO - Sci Total Environ. 2014 Jan 1;466-467:524-32. doi: 10.1016/j.scitotenv.2013.07.058. Epub 2013 Aug 10.