PMID- 24509565 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20141001 LR - 20211021 IS - 2045-2322 (Electronic) IS - 2045-2322 (Linking) VI - 4 DP - 2014 Feb 10 TI - Metal-semiconductor barrier modulation for high photoresponse in transition metal dichalcogenide field effect transistors. PG - 4041 LID - 10.1038/srep04041 [doi] LID - 4041 AB - A gate-controlled metal-semiconductor barrier modulation and its effect on carrier transport were investigated in two-dimensional (2D) transition metal dichalcogenide (TMDC) field effect transistors (FETs). A strong photoresponse was observed in both unipolar MoS2 and ambipolar WSe2 FETs (i) at the high drain voltage due to a high electric field along the channel for separating photo-excited charge carriers and (ii) at the certain gate voltage due to the optimized barriers for the collection of photo-excited charge carriers at metal contacts. The effective barrier height between Ti/Au and TMDCs was estimated by a low temperature measurement. An ohmic contact behavior and drain-induced barrier lowering (DIBL) were clearly observed in MoS2 FET. In contrast, a Schottky-to-ohmic contact transition was observed in WSe2 FET as the gate voltage increases, due to the change of majority carrier transport from holes to electrons. The gate-dependent barrier modulation effectively controls the carrier transport, demonstrating its great potential in 2D TMDCs for electronic and optoelectronic applications. FAU - Li, Hua-Min AU - Li HM AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Lee, Dae-Yeong AU - Lee DY AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Choi, Min Sup AU - Choi MS AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Qu, Deshun AU - Qu D AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Liu, Xiaochi AU - Liu X AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Ra, Chang-Ho AU - Ra CH AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. FAU - Yoo, Won Jong AU - Yoo WJ AD - Samsung-SKKU Graphene Center (SSGC), SKKU Advanced Institute of Nano Technology (SAINT), Department of Nano Science and Technology, Sungkyunkwan University, 2066 Seobu-ro, Jangan-gu, Suwon 440-746, Korea. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20140210 PL - England TA - Sci Rep JT - Scientific reports JID - 101563288 PMC - PMC3918928 EDAT- 2014/02/11 06:00 MHDA- 2014/02/11 06:01 PMCR- 2014/02/10 CRDT- 2014/02/11 06:00 PHST- 2013/08/02 00:00 [received] PHST- 2014/01/24 00:00 [accepted] PHST- 2014/02/11 06:00 [entrez] PHST- 2014/02/11 06:00 [pubmed] PHST- 2014/02/11 06:01 [medline] PHST- 2014/02/10 00:00 [pmc-release] AID - srep04041 [pii] AID - 10.1038/srep04041 [doi] PST - epublish SO - Sci Rep. 2014 Feb 10;4:4041. doi: 10.1038/srep04041.