PMID- 24967616 OWN - NLM STAT- MEDLINE DCOM- 20150511 LR - 20140722 IS - 1520-5827 (Electronic) IS - 0743-7463 (Linking) VI - 30 IP - 28 DP - 2014 Jul 22 TI - Functional polymer sheet patterning using microfluidics. PG - 8637-44 LID - 10.1021/la501723n [doi] AB - Poly(dimethylsiloxane) (PDMS)-based microfluidics provide a novel approach to advanced material synthesis. While PDMS has been successfully used in a wide range of industrial applications, due to the weak mechanical property channels generally possess low aspect ratios (AR) and thus produce microparticles with similarly low ARs. By increasing the channel width to nearly 1 cm, AR to 267, and implementing flow lithography, we were able to establish the slit-channel lithography. Not only does this allow us to synthesize sheet materials bearing multiscale features and tunable chemical anisotropy but it also allows us to fabricate functional layered sheet structures in a one-step, high-throughput fashion. We showcased the technique's potential role in various applications, such as the synthesis of planar material with micro- and nanoscale features, surface morphologies, construction of tubular and 3D layered hydrogel tissue scaffolds, and one-step formation of radio frequency identification (RFID) tags. The method introduced offers a novel route to functional sheet material synthesis and sheet system fabrication. FAU - Li, Minggan AU - Li M AD - Department of Chemical Engineering, Ryerson University , 350 Victoria Street, Toronto, Ontario M5B 2K3, Canada. FAU - Humayun, Mouhita AU - Humayun M FAU - Kozinski, Janusz A AU - Kozinski JA FAU - Hwang, Dae Kun AU - Hwang DK LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20140708 PL - United States TA - Langmuir JT - Langmuir : the ACS journal of surfaces and colloids JID - 9882736 RN - 0 (Dimethylpolysiloxanes) RN - 0 (Polymers) RN - 63148-62-9 (baysilon) SB - IM MH - Dimethylpolysiloxanes/chemistry MH - Microfluidics/*methods MH - Polymers/*chemistry EDAT- 2014/06/27 06:00 MHDA- 2015/05/12 06:00 CRDT- 2014/06/27 06:00 PHST- 2014/06/27 06:00 [entrez] PHST- 2014/06/27 06:00 [pubmed] PHST- 2015/05/12 06:00 [medline] AID - 10.1021/la501723n [doi] PST - ppublish SO - Langmuir. 2014 Jul 22;30(28):8637-44. doi: 10.1021/la501723n. Epub 2014 Jul 8.