PMID- 25382854 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20150331 LR - 20141210 IS - 1944-8252 (Electronic) IS - 1944-8244 (Linking) VI - 6 IP - 23 DP - 2014 Dec 10 TI - Growth of large-scale and thickness-modulated MoS(2) nanosheets. PG - 21215-22 LID - 10.1021/am506198b [doi] AB - Two-dimensional MoS2 is a promising material for next-generation electronic and optoelectronic devices due to its unique electrical and optical properties including the band gap modulation with film thickness. Although MoS2 has shown excellent properties, wafer-scale production with layer control from single to few layers has yet to be demonstrated. The present study explored the large-scale and thickness-modulated growth of atomically thin MoS2 on Si/SiO2 substrates using a two-step sputtering-CVD method. Our process exhibited wafer-scale fabrication and successful thickness modulation of MoS2 layers from monolayer (0.72 nm) to multilayer (12.69 nm) with high uniformity. Electrical measurements on MoS2 field effect transistors (FETs) revealed a p-type semiconductor behavior with much higher field effect mobility and current on/off ratio as compared to previously reported CVD grown MoS2-FETs and amorphous silicon (a-Si) thin film transistors. Our results show that sputter-CVD is a viable method to synthesize large-area, high-quality, and layer-controlled MoS2 that can be adapted in conventional Si-based microfabrication technology and future flexible, high-temperature, and radiation hard electronics/optoelectronics. FAU - Choudhary, Nitin AU - Choudhary N AD - Department of Materials Science and Engineering, University of North Texas , Denton, Texas 76207, United States. FAU - Park, Juhong AU - Park J FAU - Hwang, Jun Yeon AU - Hwang JY FAU - Choi, Wonbong AU - Choi W LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20141126 PL - United States TA - ACS Appl Mater Interfaces JT - ACS applied materials & interfaces JID - 101504991 OTO - NOTNLM OT - MoS2 OT - PVD-CVD OT - field effect transistors OT - thin films EDAT- 2014/11/11 06:00 MHDA- 2014/11/11 06:01 CRDT- 2014/11/11 06:00 PHST- 2014/11/11 06:00 [entrez] PHST- 2014/11/11 06:00 [pubmed] PHST- 2014/11/11 06:01 [medline] AID - 10.1021/am506198b [doi] PST - ppublish SO - ACS Appl Mater Interfaces. 2014 Dec 10;6(23):21215-22. doi: 10.1021/am506198b. Epub 2014 Nov 26.