PMID- 25818091 OWN - NLM STAT- MEDLINE DCOM- 20160108 LR - 20181202 IS - 1873-6424 (Electronic) IS - 0269-7491 (Linking) VI - 202 DP - 2015 Jul TI - Estimating dry deposition and gas/particle partition coefficients of neutral poly-/perfluoroalkyl substances in northern German coast. PG - 120-5 LID - S0269-7491(15)00159-1 [pii] LID - 10.1016/j.envpol.2015.03.029 [doi] AB - Dry deposition fluxes of 12 neutral poly-/perfluoroalkyl substances (PFASs) were estimated at Busum located in northern German coast, and their gas/particle partition coefficients were predicted by employing the polyparameter linear free energy relationships (PP-LFERs). The gas deposition flux, particle deposition flux and total (gas + particle) flux of the 12 PFASs during sampling periods were 1088 +/- 611, 189 +/- 75 and 1277 +/- 627 pg/(m(2) d), respectively. The gas deposition of PFASs played a key role during deposition to marine ecosystem. Sensitivity analysis showed that wind speed was the most sensitive parameter for gas deposition fluxes. Good agreements (within 1 log unit) were observed between the measured gas/particle partitioning data of PFASs and the predicted partition coefficients using PP-LFERs, indicating the model can reliably predict the gas/particle partitioning behaviors of atmospheric neutral PFASs. CI - Copyright (c) 2015 Elsevier Ltd. All rights reserved. FAU - Wang, Zhen AU - Wang Z AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany; National Marine Environmental Monitoring Center, Dalian 116023, China. FAU - Xie, Zhiyong AU - Xie Z AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany. Electronic address: zhiyong.xie@hzg.de. FAU - Moller, Axel AU - Moller A AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany. FAU - Mi, Wenying AU - Mi W AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany. FAU - Wolschke, Hendrik AU - Wolschke H AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany. FAU - Ebinghaus, Ralf AU - Ebinghaus R AD - Helmholtz-Zentrum Geesthacht, Institute for Coastal Research, 21502 Geesthacht, Germany. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20150326 PL - England TA - Environ Pollut JT - Environmental pollution (Barking, Essex : 1987) JID - 8804476 RN - 0 (Air Pollutants) RN - 0 (Fluorocarbons) RN - 0 (Gases) RN - 0 (Particulate Matter) RN - 0 (Volatile Organic Compounds) RN - 0 (Water Pollutants, Chemical) SB - IM MH - Air Pollutants/*analysis MH - Environmental Monitoring/*methods MH - Fluorocarbons/*analysis MH - Gases/chemistry MH - Germany MH - Models, Theoretical MH - Particulate Matter/*analysis MH - Volatile Organic Compounds/*analysis MH - Water Pollutants, Chemical/*analysis OTO - NOTNLM OT - 8:2 FTOH OT - Gas diffusive deposition OT - Gas/particle partition coefficients OT - PFASs OT - PP-LFERs EDAT- 2015/03/31 06:00 MHDA- 2016/01/09 06:00 CRDT- 2015/03/31 06:00 PHST- 2015/01/23 00:00 [received] PHST- 2015/03/19 00:00 [revised] PHST- 2015/03/23 00:00 [accepted] PHST- 2015/03/31 06:00 [entrez] PHST- 2015/03/31 06:00 [pubmed] PHST- 2016/01/09 06:00 [medline] AID - S0269-7491(15)00159-1 [pii] AID - 10.1016/j.envpol.2015.03.029 [doi] PST - ppublish SO - Environ Pollut. 2015 Jul;202:120-5. doi: 10.1016/j.envpol.2015.03.029. Epub 2015 Mar 26.