PMID- 26267210
OWN - NLM
STAT- PubMed-not-MEDLINE
DCOM- 20151020
LR  - 20150813
IS  - 1948-7185 (Electronic)
IS  - 1948-7185 (Linking)
VI  - 6
IP  - 15
DP  - 2015 Aug 6
TI  - Dynamics of a One-Dimensional Holstein Polaron with the Hierarchical Equations of 
      Motion Approach.
PG  - 3110-5
LID - 10.1021/acs.jpclett.5b01368 [doi]
AB  - Dynamics of a one-dimensional Holstein molecular crystal model is investigated by 
      making use of the hierarchical equations of motion (HEOM) introduced by Tanimura 
      and Kubo [J. Phys. Soc. Jpn. 1989, 104, 101]. Our extended, numerically exact 
      HEOM approach is capable of treating exciton-phonon coupling in a nonperturbative 
      manner and is applicable to any temperature. It is revealed that strong exciton 
      phonon coupling leads to excitonic localization, while a large exciton transfer 
      integral facilitates exciton transport. Temperature effects on excitonic 
      scattering have also been examined. A proof of concept, our work also serves as a 
      benchmark for future comparisons with other numerical approaches to Holstein 
      polaron dynamics.
FAU - Chen, Lipeng
AU  - Chen L
AD  - Division of Materials Science, Nanyang Technological University, 50 Nanyang 
      Avenue, Singapore 639798.
AD  - Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 
      606-8502, Japan.
FAU - Zhao, Yang
AU  - Zhao Y
AD  - Division of Materials Science, Nanyang Technological University, 50 Nanyang 
      Avenue, Singapore 639798.
AD  - Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 
      606-8502, Japan.
FAU - Tanimura, Yoshitaka
AU  - Tanimura Y
AD  - Division of Materials Science, Nanyang Technological University, 50 Nanyang 
      Avenue, Singapore 639798.
AD  - Department of Chemistry, Graduate School of Science, Kyoto University, Kyoto 
      606-8502, Japan.
LA  - eng
PT  - Journal Article
DEP - 20150728
PL  - United States
TA  - J Phys Chem Lett
JT  - The journal of physical chemistry letters
JID - 101526034
OTO - NOTNLM
OT  - HEOM
OT  - Holstein model
OT  - exciton scattering
OT  - exciton transport
OT  - exciton-phonon coupling
EDAT- 2015/08/13 06:00
MHDA- 2015/08/13 06:01
CRDT- 2015/08/13 06:00
PHST- 2015/08/13 06:00 [entrez]
PHST- 2015/08/13 06:00 [pubmed]
PHST- 2015/08/13 06:01 [medline]
AID - 10.1021/acs.jpclett.5b01368 [doi]
PST - ppublish
SO  - J Phys Chem Lett. 2015 Aug 6;6(15):3110-5. doi: 10.1021/acs.jpclett.5b01368. Epub 
      2015 Jul 28.