PMID- 28988083 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20180316 LR - 20180316 IS - 1879-1026 (Electronic) IS - 0048-9697 (Linking) VI - 615 DP - 2018 Feb 15 TI - High-resolution sedimentary records of some organochlorine pesticides in Yamzho Yumco Lake of the Tibetan Plateau: Concentration and composition. PG - 469-475 LID - S0048-9697(17)32633-5 [pii] LID - 10.1016/j.scitotenv.2017.09.282 [doi] AB - Sediment cores from lakes have been used to reconstruct the historic deposition of persistent organic pollutants (POPs), especially in remote alpine areas. To reconstruct the deposition history of organochlorine pesticides (OCPs) in the Tibetan Plateau (TP), two sediment cores from Yamzho Yumco Lake were drilled and dated with high-resolution, from which 23 OCPs were analyzed in greater detail. Regarding several legacy compounds, concentration peaks in the cores were observed in the 1970s, corresponding to the heavy usage of these compounds around the world. In addition, another peak was found at the end of the 1990s, which was explained as the addition of OCPs released from melting glaciers or the cryosphere due to global warming. Furthermore, it was found that the transformation or degradation of OCPs after deposition in the lake was limited by comparing the values of isomeric ratios at different times, such as (DDD+DDE)/ summation operatorDDTs, o,p'-DDT/p,p'-DDT and beta-HCH/ summation operatorHCHs. Such results ensure that the detected OCPs in the lake sediments really reflect their characteristics at the time of deposition. On the other hand, weak environmental self-purification of the OCPs made them last longer in the TP than in other regions. Reasonably, the fragile ecological environment of the TP would be threatened not only by legacy POPs that remain in the sediments and soils but also by POPs released from melting glaciers or the cryosphere in the next few decades under the influence of global warming. Our research provides an insight into the influence of global warming and glacial melting on the environment of the TP, and further work to gain a better understanding of the environmental processes of POPs in the TP is ongoing. CI - Copyright (c) 2017 Elsevier B.V. All rights reserved. FAU - Sun, Yong AU - Sun Y AD - State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Beijing 100083, China; School of the Earth Sciences and Resources, China University of Geosciences, Beijing 100083, China. FAU - Yuan, Guo-Li AU - Yuan GL AD - State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Beijing 100083, China; School of the Earth Sciences and Resources, China University of Geosciences, Beijing 100083, China. Electronic address: yuangl@cugb.edu.cn. FAU - Li, Jun AU - Li J AD - School of the Earth Sciences and Resources, China University of Geosciences, Beijing 100083, China. FAU - Tang, Jianhui AU - Tang J AD - Key Laboratory of Coastal Environmental Processes and Ecological Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai 264003, China. FAU - Wang, Gen-Hou AU - Wang GH AD - School of the Earth Sciences and Resources, China University of Geosciences, Beijing 100083, China. LA - eng PT - Journal Article DEP - 20171005 PL - Netherlands TA - Sci Total Environ JT - The Science of the total environment JID - 0330500 OTO - NOTNLM OT - Glacial melting OT - Global warming OT - High-resolution dating OT - Organochlorine pesticides OT - Sediment cores EDAT- 2017/10/11 06:00 MHDA- 2017/10/11 06:01 CRDT- 2017/10/09 06:00 PHST- 2017/07/23 00:00 [received] PHST- 2017/09/25 00:00 [revised] PHST- 2017/09/26 00:00 [accepted] PHST- 2017/10/11 06:00 [pubmed] PHST- 2017/10/11 06:01 [medline] PHST- 2017/10/09 06:00 [entrez] AID - S0048-9697(17)32633-5 [pii] AID - 10.1016/j.scitotenv.2017.09.282 [doi] PST - ppublish SO - Sci Total Environ. 2018 Feb 15;615:469-475. doi: 10.1016/j.scitotenv.2017.09.282. Epub 2017 Oct 5.