PMID- 29324383 OWN - NLM STAT- MEDLINE DCOM- 20180613 LR - 20180613 IS - 1879-1298 (Electronic) IS - 0045-6535 (Linking) VI - 196 DP - 2018 Apr TI - The influence of algal organic matter produced by Microcystis aeruginosa on coagulation-ultrafiltration treatment of natural organic matter. PG - 418-428 LID - S0045-6535(17)32176-8 [pii] LID - 10.1016/j.chemosphere.2017.12.198 [doi] AB - Cyanobacterial bloom causes the release of algal organic matter (AOM), which inevitably affects the treatment processes of natural organic matter (NOM). This study works on treating micro-polluted surface water (SW) by emerging coagulant, namely titanium sulfate (Ti(SO(4))(2)), followed by Low Pressure Ultrafiltration (LPUF) technology. In particular, we explored the respective influence of extracellular organic matter (EOM) and intracellular organic matter (IOM) on synergetic EOM-NOM/IOM-NOM removal, functional mechanisms and subsequent filtration performance. Results show that the IOM inclusion in surface water body facilitated synergic IOM-NOM composite pollutants removal by Ti(SO(4))(2), wherein loosely-aggregated flocs were produced, resulting in floc cake layer with rich porosity and permeability during LPUF. On the contrary, the surface water invaded by EOM pollutants increased Ti(SO(4))(2) coagulation burden, with substantially deteriorated both UV(254)-represented and dissolved organic matter (DOC) removal. Corresponded with the weak Ti(SO(4))(2) coagulation for EOM-NOM removal was the resultant serious membrane fouling during LPUF procedure, wherein dense cake layer was formed due to the compact structure of flocs. Although the IOM enhanced NOM removal with reduced Ti(SO(4))(2) dose and yielded mitigated membrane fouling, larger percentage of irreversible fouling was seen than NOM and EOM-NOM cases, which was most likely due to the substances with small molecular weight, such as microcystin, adhering in membrane pores. This research would provide theoretical basis for dose selection and process design during AOM-NOM water treatment. CI - Copyright (c) 2018 Elsevier Ltd. All rights reserved. FAU - Xu, Jie AU - Xu J AD - Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, No.27 Shanda South Road, Jinan, 250100, People's Republic of China. FAU - Zhao, Yanxia AU - Zhao Y AD - Key Laboratory for Special Functional Aggregated Materials of Education Ministry, School of Chemistry and Chemical Engineering, Shandong University, Jinan, 250100, People's Republic of China; Environmental Engineering Research Centre, Department of Civil Engineering, The University of Hong Kong, Pokfulam, Hong Kong Special Administrative Region. Electronic address: zhaodian419@163.com. FAU - Gao, Baoyu AU - Gao B AD - Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, No.27 Shanda South Road, Jinan, 250100, People's Republic of China. Electronic address: baoyugao_sdu@aliyun.com. FAU - Han, Songlin AU - Han S AD - Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, No.27 Shanda South Road, Jinan, 250100, People's Republic of China. FAU - Zhao, Qian AU - Zhao Q AD - Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, No.27 Shanda South Road, Jinan, 250100, People's Republic of China. FAU - Liu, Xiaoli AU - Liu X AD - Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, No.27 Shanda South Road, Jinan, 250100, People's Republic of China. LA - eng PT - Journal Article DEP - 20180105 PL - England TA - Chemosphere JT - Chemosphere JID - 0320657 RN - 0 (Membranes, Artificial) RN - D1JT611TNE (Titanium) SB - IM MH - Membranes, Artificial MH - Microcystis/*metabolism MH - Permeability MH - Titanium MH - Ultrafiltration/*methods MH - Water Purification/*methods OTO - NOTNLM OT - Algal organic matter OT - Coagulation OT - Membrane fouling OT - Natural organic matter OT - Titanium sulfate EDAT- 2018/01/13 06:00 MHDA- 2018/06/14 06:00 CRDT- 2018/01/12 06:00 PHST- 2017/09/15 00:00 [received] PHST- 2017/12/29 00:00 [revised] PHST- 2017/12/31 00:00 [accepted] PHST- 2018/01/13 06:00 [pubmed] PHST- 2018/06/14 06:00 [medline] PHST- 2018/01/12 06:00 [entrez] AID - S0045-6535(17)32176-8 [pii] AID - 10.1016/j.chemosphere.2017.12.198 [doi] PST - ppublish SO - Chemosphere. 2018 Apr;196:418-428. doi: 10.1016/j.chemosphere.2017.12.198. Epub 2018 Jan 5.