PMID- 29557788 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20191120 IS - 1361-6528 (Electronic) IS - 0957-4484 (Linking) VI - 29 IP - 23 DP - 2018 Jun 8 TI - Spectrally-resolved internal quantum efficiency and carrier dynamics of semipolar [Formula: see text] core-shell triangular nanostripe GaN/InGaN LEDs. PG - 235206 LID - 10.1088/1361-6528/aab82e [doi] AB - We investigate the spectrally resolved internal quantum efficiency (IQE) and carrier dynamics in semipolar [Formula: see text] core-shell triangular nanostripe light-emitting diodes (TLEDs) using temperature-dependent photoluminescence (TDPL) and time-resolved photoluminescence (TRPL) at various excitation energy densities. Using electroluminescence, photoluminescence, and cathodoluminescence measurements, we verify the origins of the broad emission spectra from the nanostructures and confirm that localized regions of high-indium-content InGaN exist along the apex of the nanostructures. Spectrally resolved IQE measurements are then performed, with the spectra integrated from 400-450 nm and 450-500 nm to obtain the IQE of the QWs mainly near the sidewalls and apex of the TLEDs, respectively. TDPL and TRPL are used to decouple the radiative and non-radiative carrier lifetimes for different regions of the emission spectra. We observe that the IQE is higher for the spectral region between 450 nm and 500 nm compared to the IQE between 400 and 450 nm. This result is in contrast to the typical observation that the IQE of planar GaN-based LEDs is lower for longer wavelengths (i.e., higher indium contents). We also observe a longer non-radiative recombination lifetime for the longer wavelength portion of the spectrum. Several explanations are proposed for the improved IQE and longer non-radiative lifetime observed near the apex of the nanostructures. The results show that nanostructures may be leveraged to design more efficient green LEDs, potentially addressing a long-standing challenge in GaN-based materials. FAU - Okur, Serdal AU - Okur S AD - Center for High Technology Materials, University of New Mexico, Albuquerque, United States of America. FAU - Rishinaramangalam, Ashwin K AU - Rishinaramangalam AK FAU - Mishkat-Ul-Masabih, Saadat AU - Mishkat-Ul-Masabih S FAU - Nami, Mohsen AU - Nami M FAU - Liu, Sheng AU - Liu S FAU - Brener, Igal AU - Brener I FAU - Brueck, Steven R J AU - Brueck SRJ FAU - Feezell, Daniel F AU - Feezell DF LA - eng PT - Journal Article DEP - 20180320 PL - England TA - Nanotechnology JT - Nanotechnology JID - 101241272 EDAT- 2018/03/21 06:00 MHDA- 2018/03/21 06:01 CRDT- 2018/03/21 06:00 PHST- 2018/03/21 06:00 [pubmed] PHST- 2018/03/21 06:01 [medline] PHST- 2018/03/21 06:00 [entrez] AID - 10.1088/1361-6528/aab82e [doi] PST - ppublish SO - Nanotechnology. 2018 Jun 8;29(23):235206. doi: 10.1088/1361-6528/aab82e. Epub 2018 Mar 20.