PMID- 29687709 OWN - NLM STAT- MEDLINE DCOM- 20190917 LR - 20221207 IS - 1520-5851 (Electronic) IS - 0013-936X (Linking) VI - 52 IP - 11 DP - 2018 Jun 5 TI - Origin and Radiative Forcing of Black Carbon Aerosol: Production and Consumption Perspectives. PG - 6380-6389 LID - 10.1021/acs.est.8b01873 [doi] AB - Air pollution, a threat to air quality and human health, has attracted ever-increasing attention in recent years. In addition to having local influence, air pollutants can also travel the globe via atmospheric circulation and international trade. Black carbon (BC), emitted from incomplete combustion, is a unique but representative particulate pollutant. This study tracked down the BC aerosol and its direct radiative forcing to the emission sources and final consumers using the global chemical transport model (MOZART-4), the rapid radiative transfer model for general circulation simulations (RRTM), and a multiregional input-output analysis (MRIO). BC was physically transported (i.e., atmospheric transport) from western to eastern countries in the midlatitude westerlies, but its magnitude is near an order of magnitude higher if the virtual flow embodied in international trade is considered. The transboundary effects on East and South Asia by other regions increased from about 3% (physical transport only) to 10% when considering both physical and virtual transport. The influence efficiency on East Asia was also large because of the comparatively large emission intensity and emission-intensive exports (e.g., machinery and equipment). The radiative forcing in Africa imposed by consumption from Europe, North America, and East Asia (0.01 Wm(-2)) was even larger than the total forcing in North America. Understanding the supply chain and incorporating both atmospheric and virtual transport may improve multilateral cooperation on air pollutant mitigation both domestically and internationally. FAU - Meng, Jing AU - Meng J AUID- ORCID: 0000-0001-8708-0485 AD - Department of Politics and International Studies , University of Cambridge , Cambridge CB3 9DT , U.K. AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. AD - Cambridge Center for Environment, Energy and Natural Resource Governance, Department of Land Economy , University of Cambridge , Cambridge CB3 9EP , U.K. FAU - Liu, Junfeng AU - Liu J AUID- ORCID: 0000-0002-7199-6357 AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. FAU - Yi, Kan AU - Yi K AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. FAU - Yang, Haozhe AU - Yang H AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. FAU - Guan, Dabo AU - Guan D FAU - Liu, Zhu AU - Liu Z FAU - Zhang, Jiachen AU - Zhang J AD - Department of Civil and Environmental Engineering , University of Southern California , Los Angeles , California 90089 , United States. FAU - Ou, Jiamin AU - Ou J FAU - Dorling, Stephen AU - Dorling S FAU - Mi, Zhifu AU - Mi Z AD - Bartlett School of Construction and Project Management , University College London , London WC1E 7HB , U.K. FAU - Shen, Huizhong AU - Shen H AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. FAU - Zhong, Qirui AU - Zhong Q AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. FAU - Tao, Shu AU - Tao S AUID- ORCID: 0000-0002-7374-7063 AD - Laboratory for Earth Surface Processes, College of Urban and Environmental Sciences , Peking University , Beijing 100871 , China. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20180514 PL - United States TA - Environ Sci Technol JT - Environmental science & technology JID - 0213155 RN - 0 (Aerosols) RN - 0 (Air Pollutants) RN - 7440-44-0 (Carbon) SB - IM MH - Aerosols MH - Africa MH - *Air Pollutants MH - Asia MH - Carbon MH - Europe MH - Asia, Eastern MH - Humans MH - North America EDAT- 2018/04/25 06:00 MHDA- 2019/09/19 06:00 CRDT- 2018/04/25 06:00 PHST- 2018/04/25 06:00 [pubmed] PHST- 2019/09/19 06:00 [medline] PHST- 2018/04/25 06:00 [entrez] AID - 10.1021/acs.est.8b01873 [doi] PST - ppublish SO - Environ Sci Technol. 2018 Jun 5;52(11):6380-6389. doi: 10.1021/acs.est.8b01873. Epub 2018 May 14.