PMID- 30529855
OWN - NLM
STAT- MEDLINE
DCOM- 20190221
LR  - 20231213
IS  - 1879-1298 (Electronic)
IS  - 0045-6535 (Linking)
VI  - 219
DP  - 2019 Mar
TI  - Preparation of magnetic polyimide@ Mg-Fe layered double hydroxides core-shell 
      composite for effective removal of various organic contaminants from aqueous 
      solution.
PG  - 66-75
LID - S0045-6535(18)32316-6 [pii]
LID - 10.1016/j.chemosphere.2018.11.209 [doi]
AB  - In this work, a novel core-shell structured magnetic polyimide@layered double 
      oxides (LDO) composites coating a porous polyimide (PI)-coated Fe(3)O(4) magnetic 
      core and layered double hydroxide (LDH) has been successfully synthesized by 
      solve-thermal synthesis and co-precipitation process. The magnetic PI@LDO 
      composites were characterized by scanning and transmission electron microscopy 
      (SEM and TEM), X-ray diffraction (XRD), thermogravimetry analysis (TGA) and 
      magnetic properties analysis. The composite materials displayed core-shell 
      structure with flower-like morphology. The magnetic PI@LDO composites were 
      applied to remove tetracycline (TC), 2,4-dichlorophenol (2,4-DCP) and glyphosate 
      (GP) from aqueous solution. The action pH value was ranged from 5 to 9 for TC and 
      GP and 3 to 7 for 2,4-DCP, respectively. Cl(-) showed a weak competitive 
      adsorption effect to TC, 2, 4-DCP and GP. In addition, the presence of humic acid 
      (HA) could slightly reduce the adsorption capacity of magnetic PI@LDO composites. 
      The adsorption process could be well described by pseudo-second-order model for 
      TC and GP, while pseudo-first-order model for 2,4-DCP. The experimental data of 
      TC and 2,4-DCP could be fitted better with Freundlich model, while that of GP 
      were fitted better with Langmuir model. The adsorptions of TC, 2,4-DCP and GP 
      were both spontaneous and endothermic. The adsorption capacity decreased slightly 
      after adsorption-desorption cycles repeated five times. This study demonstrated 
      that magnetic PI@LDO exhibited great potential to be a mild and cost-effective 
      adsorbent for the removal of various organic contaminants from wastewater.
CI  - Copyright (c) 2018 Elsevier Ltd. All rights reserved.
FAU - Wu, Hanjun
AU  - Wu H
AD  - School of Chemistry and Environmental Engineering, Wuhan Institute of Technology, 
      Wuhan, 430074, Hubei, China; Faculty of Materials Science and Chemistry, China 
      University of Geosciences, Wuhan, 430074, Hubei, China.
FAU - Zhang, Huali
AU  - Zhang H
AD  - School of Chemistry and Environmental Engineering, Wuhan Institute of Technology, 
      Wuhan, 430074, Hubei, China.
FAU - Zhang, Weijun
AU  - Zhang W
AD  - School of Environmental Studies, China University of Geosciences, Wuhan, 430074, 
      Hubei, China. Electronic address: zhangweijun@cug.edu.cn.
FAU - Yang, Xiaofang
AU  - Yang X
AD  - State Key Laboratory of Environmental Aquatic Chemistry, Research Center for 
      Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, China.
FAU - Zhou, Hong
AU  - Zhou H
AD  - School of Chemistry and Environmental Engineering, Wuhan Institute of Technology, 
      Wuhan, 430074, Hubei, China.
FAU - Pan, Zhiquan
AU  - Pan Z
AD  - School of Chemistry and Environmental Engineering, Wuhan Institute of Technology, 
      Wuhan, 430074, Hubei, China.
FAU - Wang, Dongsheng
AU  - Wang D
AD  - Faculty of Materials Science and Chemistry, China University of Geosciences, 
      Wuhan, 430074, Hubei, China; State Key Laboratory of Environmental Aquatic 
      Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of 
      Sciences, Beijing, 100085, China.
LA  - eng
PT  - Journal Article
DEP - 20181203
PL  - England
TA  - Chemosphere
JT  - Chemosphere
JID - 0320657
RN  - 0 (Chlorophenols)
RN  - 0 (Humic Substances)
RN  - 0 (Hydroxides)
RN  - 0 (Imides)
RN  - 0 (Oxides)
RN  - F8VB5M810T (Tetracycline)
RN  - R669TG1950 (2,4-dichlorophenol)
RN  - TE7660XO1C (Glycine)
SB  - IM
MH  - Adsorption
MH  - Chlorophenols/isolation & purification
MH  - Glycine/analogs & derivatives/isolation & purification
MH  - Humic Substances
MH  - Hydroxides/*chemistry
MH  - Imides/chemistry
MH  - *Magnetics
MH  - *Oxides/chemistry
MH  - Tetracycline/chemistry
MH  - Water Purification/*methods
MH  - Glyphosate
OTO - NOTNLM
OT  - Adsoption behavior
OT  - Core-shell structure
OT  - Magnetic polyimide@ layered double oxides composites
OT  - Organic contaminants
OT  - Regeneration
EDAT- 2018/12/12 06:00
MHDA- 2019/02/23 06:00
CRDT- 2018/12/12 06:00
PHST- 2018/08/03 00:00 [received]
PHST- 2018/11/24 00:00 [revised]
PHST- 2018/11/29 00:00 [accepted]
PHST- 2018/12/12 06:00 [pubmed]
PHST- 2019/02/23 06:00 [medline]
PHST- 2018/12/12 06:00 [entrez]
AID - S0045-6535(18)32316-6 [pii]
AID - 10.1016/j.chemosphere.2018.11.209 [doi]
PST - ppublish
SO  - Chemosphere. 2019 Mar;219:66-75. doi: 10.1016/j.chemosphere.2018.11.209. Epub 
      2018 Dec 3.