PMID- 30573074
OWN - NLM
STAT- MEDLINE
DCOM- 20190111
LR  - 20190111
IS  - 1001-0742 (Print)
IS  - 1001-0742 (Linking)
VI  - 77
DP  - 2019 Mar
TI  - Efficient capture of aqueous humic acid using a functionalized stereoscopic 
      porous activated carbon based on poly(acrylic acid)/food-waste hydrogel.
PG  - 104-114
LID - S1001-0742(18)30402-9 [pii]
LID - 10.1016/j.jes.2018.06.019 [doi]
AB  - Stereoscopic porous carbons have shown good potential in humic acid (HA) removal. 
      In this work, a novel stereoscopic porous activated carbon (SPAC) was designed 
      and synthesized via the self-assembly of a hydrogel based on food waste during 
      in-situ polymerization, vacuum drying, carbonization, and activation. Then, the 
      SPAC was functionalized with 3-aminopropyltriethoxysilane (APTES) and the 
      adsorption behavior of the modified SPAC (SPAC-NH(2)) was studied systematically. 
      The effects of pH, contact time, initial concentration of HA, and adsorbent dose 
      were investigated, showing that optimal HA removal efficiency (>98.0%) could be 
      achieved at an initial HA concentration of 100 mg/L. The experimental adsorption 
      isotherm data was fitted to the Langmuir model with a maximum adsorption capacity 
      of 156.0 mg HA/g SPAC-NH(2). Analysis of the mechanism indicated that the removal 
      of HA was mainly realized through the amidization reaction between the COOH 
      groups of HA and the NH(2) groups of APTES. All of the above results showed that 
      SPAC-NH(2) powder is an efficient, eco-friendly, and reusable adsorbent which is 
      suitable for the removal of HA from wastewater.
CI  - Copyright (c) 2018. Published by Elsevier B.V.
FAU - Zhou, Tao
AU  - Zhou T
AD  - The State Key Laboratory of Pollution Control and Resource Reuse, School of 
      Environmental Science and Engineering, Tongji University, Shanghai 200092, China.
FAU - Zhao, Xin
AU  - Zhao X
AD  - Shanghai Chengpei Enterprise Management Consulting Co., Ltd., Shanghai 200000, 
      China.
FAU - Wu, Shuya
AU  - Wu S
AD  - The State Key Laboratory of Pollution Control and Resource Reuse, School of 
      Environmental Science and Engineering, Tongji University, Shanghai 200092, China.
FAU - Su, Lianghu
AU  - Su L
AD  - Nanjing Institute of Environmental Sciences, Ministry of Environmental 
      Protection, Nanjing 210042, China.
FAU - Zhao, Youcai
AU  - Zhao Y
AD  - The State Key Laboratory of Pollution Control and Resource Reuse, School of 
      Environmental Science and Engineering, Tongji University, Shanghai 200092, China; 
      Shanghai Institute of Pollution Control and Ecological Security, 1515 North 
      Zhongshan Rd. (No. 2), Shanghai 200092, China. Electronic address: 
      zhaoyoucai@tongji.edu.cn.
LA  - eng
PT  - Journal Article
DEP - 20180630
PL  - Netherlands
TA  - J Environ Sci (China)
JT  - Journal of environmental sciences (China)
JID - 100967627
RN  - 0 (Acrylic Resins)
RN  - 0 (Humic Substances)
RN  - 0 (Hydrogels)
RN  - 0 (Waste Products)
RN  - 059QF0KO0R (Water)
RN  - 16291-96-6 (Charcoal)
RN  - 4Q93RCW27E (carbopol 940)
SB  - IM
MH  - Acrylic Resins/*chemistry
MH  - Adsorption
MH  - Charcoal/*chemistry
MH  - *Food
MH  - *Humic Substances
MH  - Hydrogels/*chemistry
MH  - Hydrogen-Ion Concentration
MH  - Porosity
MH  - Time Factors
MH  - *Waste Products
MH  - Water/*chemistry
OTO - NOTNLM
OT  - 3-aminopropyltriethoxysilane
OT  - Adsorption
OT  - Food waste
OT  - Humic acid
OT  - Stereoscopic porous activated carbon
EDAT- 2018/12/24 06:00
MHDA- 2019/01/12 06:00
CRDT- 2018/12/22 06:00
PHST- 2018/02/08 00:00 [received]
PHST- 2018/06/21 00:00 [revised]
PHST- 2018/06/22 00:00 [accepted]
PHST- 2018/12/22 06:00 [entrez]
PHST- 2018/12/24 06:00 [pubmed]
PHST- 2019/01/12 06:00 [medline]
AID - S1001-0742(18)30402-9 [pii]
AID - 10.1016/j.jes.2018.06.019 [doi]
PST - ppublish
SO  - J Environ Sci (China). 2019 Mar;77:104-114. doi: 10.1016/j.jes.2018.06.019. Epub 
      2018 Jun 30.