PMID- 30855970
OWN - NLM
STAT- PubMed-not-MEDLINE
LR  - 20201001
IS  - 1530-6992 (Electronic)
IS  - 1530-6984 (Linking)
VI  - 19
IP  - 4
DP  - 2019 Apr 10
TI  - Impact of Organic Molecule-Induced Charge Transfer on Operating Voltage Control 
      of Both n-MoS(2) and p-MoTe(2) Transistors.
PG  - 2456-2463
LID - 10.1021/acs.nanolett.9b00019 [doi]
AB  - Since transition metal dichalcogenide (TMD) semiconductors are found as 
      two-dimensional van der Waals materials with a discrete energy bandgap, many TMD 
      based field effect transistors (FETs) are reported as prototype devices. However, 
      overall reports indicate that threshold voltage ( V(th)) of those FETs are 
      located far away from 0 V whether the channel is p- or n-type. This definitely 
      causes high switching voltage and unintended OFF-state leakage current. Here, a 
      facile way to simultaneously modulate the V(th) of both p- and n-channel FETs 
      with TMDs is reported. The deposition of various organic small molecules on the 
      channel results in charge transfer between the organic molecule and TMD channels. 
      Especially, HAT-CN molecule is found to ideally work for both p- and n-channels, 
      shifting their V(th) toward 0 V concurrently. As a proof of concept, a 
      complementary metal oxide semiconductor (CMOS) inverter with p-MoTe(2) and 
      n-MoS(2) channels shows superior voltage gain and minimal power consumption after 
      HAT-CN deposition, compared to its initial performance. When the same TMD FETs of 
      the CMOS structure are integrated into an OLED pixel circuit for ambipolar 
      switching, the circuit with HAT-CN film demonstrates complete ON/OFF switching of 
      OLED pixel, which was not switched off without HAT-CN.
FAU - Cho, Yongjae
AU  - Cho Y
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Park, Ji Hoon
AU  - Park JH
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Kim, Minju
AU  - Kim M
AUID- ORCID: 0000-0002-7466-7129
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Jeong, Yeonsu
AU  - Jeong Y
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Yu, Sanghyuck
AU  - Yu S
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Lim, June Yeong
AU  - Lim JY
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Yi, Yeonjin
AU  - Yi Y
AUID- ORCID: 0000-0003-4944-8319
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
FAU - Im, Seongil
AU  - Im S
AUID- ORCID: 0000-0003-0723-5075
AD  - Van der Waals Materials Research Center, Department of Physics and Applied 
      Physics , Yonsei University , 50 Yonsei-ro , Seodaemun-gu , Seoul 03722 , Korea.
LA  - eng
PT  - Journal Article
PT  - Research Support, Non-U.S. Gov't
DEP - 20190313
PL  - United States
TA  - Nano Lett
JT  - Nano letters
JID - 101088070
OTO - NOTNLM
OT  - HAT-CN
OT  - TMD
OT  - charge transfer
OT  - organic molecules
OT  - threshold voltage
EDAT- 2019/03/12 06:00
MHDA- 2019/03/12 06:01
CRDT- 2019/03/12 06:00
PHST- 2019/03/12 06:00 [pubmed]
PHST- 2019/03/12 06:01 [medline]
PHST- 2019/03/12 06:00 [entrez]
AID - 10.1021/acs.nanolett.9b00019 [doi]
PST - ppublish
SO  - Nano Lett. 2019 Apr 10;19(4):2456-2463. doi: 10.1021/acs.nanolett.9b00019. Epub 
      2019 Mar 13.