PMID- 31100560
OWN - NLM
STAT- PubMed-not-MEDLINE
LR  - 20190723
IS  - 1873-3336 (Electronic)
IS  - 0304-3894 (Linking)
VI  - 375
DP  - 2019 Aug 5
TI  - Nano-sized architectural design of multi-activity graphene oxide (GO) by chemical 
      post-decoration for efficient uranium(VI) extraction.
PG  - 320-329
LID - S0304-3894(19)30531-X [pii]
LID - 10.1016/j.jhazmat.2019.05.005 [doi]
AB  - The introduction of organic groups onto graphene oxide (GO) platelets can supply 
      additional active sites for adsorption of uranium(VI) (U(VI)) to improve the 
      adsorption capacity. However, as a result of the existence of stabilizing 
      pi-conjugation system, a facile and effective modification method remains a 
      challenge. Therefore, a novel strategy is exploited by nano-sized architectural 
      design of multi-activity GO through post-decoration with amidoxime functionalized 
      diaminomaleonitrile (DM-AO). The post-modification of DM-AO successfully 
      activated the inert sites in GO platelets. Meanwhile, the amidoxime group in 
      DM-AO can improve the adsorption selectivity. Adsorption amount of U(VI) on the 
      as prepared GO-DM-AO reached at 935 mg g(-1), which is increased by 209% 
      increment compared with that of pristine GO at the same concentration. The 
      adsorption efficiency of GO-DM-AO is greatly improved, and the time to reach the 
      adsorption equilibrium is half of that of GO. Excitingly, the excellent removal 
      efficiency could still maintained even after 5 cycles of adsorption-desorption. 
      The outstanding adsorption amount, short adsorption equilibrium time, and 
      excellent removal efficiency can provide a theoretical guidance for further 
      immobilization of U(VI) from seawater.
CI  - Copyright (c) 2019 Elsevier B.V. All rights reserved.
FAU - Yang, Peipei
AU  - Yang P
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Zhang, Hongsen
AU  - Zhang H
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Liu, Qi
AU  - Liu Q
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Liu, Jingyuan
AU  - Liu J
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Chen, Rongrong
AU  - Chen R
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Yu, Jing
AU  - Yu J
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China.
FAU - Hou, Jindi
AU  - Hou J
AD  - College of Science, Harbin Engineering University, 150001, PR China.
FAU - Bai, Xuefeng
AU  - Bai X
AD  - College of Material Science and Chemical Engineering, Harbin Engineering 
      University, 150001, PR China.
FAU - Wang, Jun
AU  - Wang J
AD  - Key Laboratory of Superlight Material and Surface Technology, Ministry of 
      Education, Harbin Engineering University, 150001, PR China; College of Material 
      Science and Chemical Engineering, Harbin Engineering University, 150001, PR 
      China; Institute of Advanced Marine Materials, Harbin Engineering University, 
      150001, PR China. Electronic address: zhqw1888@sohu.com.
LA  - eng
PT  - Journal Article
DEP - 20190503
PL  - Netherlands
TA  - J Hazard Mater
JT  - Journal of hazardous materials
JID - 9422688
OTO - NOTNLM
OT  - Amidoxime functionalized
OT  - Graphene oxide
OT  - Nano-sized architectural
OT  - Uranium adsorption
EDAT- 2019/05/18 06:00
MHDA- 2019/05/18 06:01
CRDT- 2019/05/18 06:00
PHST- 2019/02/14 00:00 [received]
PHST- 2019/04/18 00:00 [revised]
PHST- 2019/05/02 00:00 [accepted]
PHST- 2019/05/18 06:00 [pubmed]
PHST- 2019/05/18 06:01 [medline]
PHST- 2019/05/18 06:00 [entrez]
AID - S0304-3894(19)30531-X [pii]
AID - 10.1016/j.jhazmat.2019.05.005 [doi]
PST - ppublish
SO  - J Hazard Mater. 2019 Aug 5;375:320-329. doi: 10.1016/j.jhazmat.2019.05.005. Epub 
      2019 May 3.