PMID- 31170625 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20201001 IS - 2589-0042 (Electronic) IS - 2589-0042 (Linking) VI - 16 DP - 2019 Jun 28 TI - Particulate Matter Capturing via Naturally Dried ZIF-8/Graphene Aerogels under Harsh Conditions. PG - 133-144 LID - S2589-0042(19)30161-0 [pii] LID - 10.1016/j.isci.2019.05.024 [doi] AB - Particulate matter (PM) pollution poses a serious threat to the environment and public health. Capture of PM is best performed at the emission source, such as car exhaust exit points, although it is a challenge for filters to work under harsh conditions of high temperatures and flow rate. Here we designed a thermally stable PM filter by in situ anchoring of zeolite imidazole framework-8 (ZIF-8) on a three-dimensional (3D) network of reduced graphene oxide aerogel (rGA) through natural drying. Owing to high specific surface area, well-connected porous network of graphene aerogel, and large number of metal sites from ZIF-8/rGA, the capture efficiencies for PM(2.5) and PM(10) are over 99.3% and 99.6%, respectively, at ambient conditions, and the efficiencies remain high in harsh conditions (PM(2.5) and PM(10): >98.8% and >99.1%, respectively, at 200 degrees C at a flow velocity of 30 L/min). The filter can be regenerated by a simple washing process. CI - Copyright (c) 2019 The Author(s). Published by Elsevier Inc. All rights reserved. FAU - Mao, Jiajun AU - Mao J AD - National Engineering Research Center of Chemical Fertilizer Catalyst (NERC-CFC), College of Chemical Engineering, Fuzhou University, Fuzhou 350116, P. R. China; National Engineering Laboratory for Modern Silk, College of Textile and Clothing Engineering, Soochow University, Suzhou 215123, P. R. China. FAU - Tang, Yuxin AU - Tang Y AD - Institute of Applied Physics and Materials Engineering, University of Macau, Macau, P. R. China. FAU - Wang, Yandong AU - Wang Y AD - Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou 215123, P. R. China. FAU - Huang, Jianying AU - Huang J AD - National Engineering Research Center of Chemical Fertilizer Catalyst (NERC-CFC), College of Chemical Engineering, Fuzhou University, Fuzhou 350116, P. R. China. FAU - Dong, Xiuli AU - Dong X AD - National Engineering Laboratory for Modern Silk, College of Textile and Clothing Engineering, Soochow University, Suzhou 215123, P. R. China. FAU - Chen, Zhong AU - Chen Z AD - School of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, 639798 Singapore, Singapore. FAU - Lai, Yuekun AU - Lai Y AD - National Engineering Research Center of Chemical Fertilizer Catalyst (NERC-CFC), College of Chemical Engineering, Fuzhou University, Fuzhou 350116, P. R. China. Electronic address: yklai@fzu.edu.cn. LA - eng PT - Journal Article DEP - 20190523 PL - United States TA - iScience JT - iScience JID - 101724038 PMC - PMC6551531 OTO - NOTNLM OT - Composite Materials OT - Materials Science OT - Nanomaterials OT - Porous Material EDAT- 2019/06/07 06:00 MHDA- 2019/06/07 06:01 PMCR- 2019/05/23 CRDT- 2019/06/07 06:00 PHST- 2019/04/03 00:00 [received] PHST- 2019/04/29 00:00 [revised] PHST- 2019/05/16 00:00 [accepted] PHST- 2019/06/07 06:00 [pubmed] PHST- 2019/06/07 06:01 [medline] PHST- 2019/06/07 06:00 [entrez] PHST- 2019/05/23 00:00 [pmc-release] AID - S2589-0042(19)30161-0 [pii] AID - 10.1016/j.isci.2019.05.024 [doi] PST - ppublish SO - iScience. 2019 Jun 28;16:133-144. doi: 10.1016/j.isci.2019.05.024. Epub 2019 May 23.