PMID- 31221380 OWN - NLM STAT- MEDLINE DCOM- 20190726 LR - 20190726 IS - 1001-0742 (Print) IS - 1001-0742 (Linking) VI - 83 DP - 2019 Sep TI - Apparent relationships between anthropogenic factors and climate change indicators and POPs deposition in a lacustrine system. PG - 174-182 LID - S1001-0742(18)33219-4 [pii] LID - 10.1016/j.jes.2019.03.024 [doi] AB - Climate change and anthropogenic activities are expected to impact the environmental behaviors and fates of persistent organic pollutants (POPs), however, quantitative studies on these combined factors are scarce. In this study, dichlorodiphenyltrichloroethane (DDTs), polycyclic aromatic hydrocarbons (PAHs), and polychlorinated biphenyls (PCBs) were used as examples to identify how and when those factors may be related to the deposition of POPs in the sediment of Lake Chaohu, China, using generalized additive models (GAMs). Three historical trends of DDT, PAH, and PCB deposition were delineated in a dated sediment core encompassing ~100 years of historical record: a steady state or gradually increasing stage, a rapidly increasing stage, and a declining stage. The GAM results showed that aquatic total phosphorus (TP) concentrations and regional GDP (anthropogenic factors) were dominant contributors to POP accumulation rates in the lake sediment. The fitted relationships between air temperature and sedimentary DDT and PAH concentrations were linear and negative, while a positive linear relationship was found for PCBs, suggesting that Lake Chaohu may have become a net source for DDTs and PAHs, and a sink for PCBs, under a progressively warming climate. CI - Copyright (c) 2019. Published by Elsevier B.V. FAU - Zhang, Hanxiao AU - Zhang H AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. FAU - Huo, Shouliang AU - Huo S AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. Electronic address: huoshouliang@126.com. FAU - Yeager, Kevin M AU - Yeager KM AD - Department Earth and Environmental Sciences, University of Kentucky, Lexington, KY 40506, USA. FAU - Li, Chaocan AU - Li C AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. FAU - Xi, Beidou AU - Xi B AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. FAU - Zhang, Jingtian AU - Zhang J AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. FAU - He, Zhuoshi AU - He Z AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. FAU - Ma, Chunzi AU - Ma C AD - State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Science, Beijing 100012, China. LA - eng PT - Journal Article DEP - 20190403 PL - Netherlands TA - J Environ Sci (China) JT - Journal of environmental sciences (China) JID - 100967627 RN - 0 (Air Pollutants) RN - 0 (Hydrocarbons, Chlorinated) RN - 0 (Polycyclic Aromatic Hydrocarbons) RN - 0 (Water Pollutants, Chemical) RN - CIW5S16655 (DDT) RN - DFC2HB4I0K (Polychlorinated Biphenyls) MH - Air Pollutants/*analysis MH - China MH - *Climate Change MH - DDT MH - *Environmental Monitoring MH - Geologic Sediments MH - Hydrocarbons, Chlorinated/analysis MH - Lakes MH - Polychlorinated Biphenyls/analysis MH - Polycyclic Aromatic Hydrocarbons/analysis MH - Water Pollutants, Chemical/analysis OTO - NOTNLM OT - Climate change OT - Generalized additive models OT - Lake sediment OT - POPs EDAT- 2019/06/22 06:00 MHDA- 2019/07/28 06:00 CRDT- 2019/06/22 06:00 PHST- 2018/11/14 00:00 [received] PHST- 2019/03/27 00:00 [revised] PHST- 2019/03/28 00:00 [accepted] PHST- 2019/06/22 06:00 [entrez] PHST- 2019/06/22 06:00 [pubmed] PHST- 2019/07/28 06:00 [medline] AID - S1001-0742(18)33219-4 [pii] AID - 10.1016/j.jes.2019.03.024 [doi] PST - ppublish SO - J Environ Sci (China). 2019 Sep;83:174-182. doi: 10.1016/j.jes.2019.03.024. Epub 2019 Apr 3.