PMID- 31408607 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20231014 IS - 1530-6992 (Electronic) IS - 1530-6984 (Print) IS - 1530-6984 (Linking) VI - 19 IP - 9 DP - 2019 Sep 11 TI - Charge-to-Spin Conversion by the Rashba-Edelstein Effect in Two-Dimensional van der Waals Heterostructures up to Room Temperature. PG - 5959-5966 LID - 10.1021/acs.nanolett.9b01611 [doi] AB - The proximity of a transition-metal dichalcogenide (TMD) to graphene imprints a rich spin texture in graphene and complements its high-quality charge/spin transport by inducing spin-orbit coupling (SOC). Rashba and valley-Zeeman SOCs are the origin of charge-to-spin conversion mechanisms such as the Rashba-Edelstein effect (REE) and spin Hall effect (SHE). In this work, we experimentally demonstrate for the first time charge-to-spin conversion due to the REE in a monolayer WS(2)-graphene van der Waals heterostructure. We measure the current-induced spin polarization up to room temperature and control it by a gate electric field. Our observation of the REE and the inverse of the effect (IREE) is accompanied by the SHE, which we discriminate by symmetry-resolved spin precession under oblique magnetic fields. These measurements also allow for the quantification of the efficiencies of charge-to-spin conversion by each of the two effects. These findings are a clear indication of induced Rashba and valley-Zeeman SOC in graphene that lead to the generation of spin accumulation and spin current without using ferromagnetic electrodes. These realizations have considerable significance for spintronic applications, providing accessible routes toward all-electrical spin generation and manipulation in two-dimensional materials. FAU - Ghiasi, Talieh S AU - Ghiasi TS AUID- ORCID: 0000-0002-3490-5356 AD - Zernike Institute for Advanced Materials , University of Groningen , Groningen , 9747 AG , The Netherlands. FAU - Kaverzin, Alexey A AU - Kaverzin AA AD - Zernike Institute for Advanced Materials , University of Groningen , Groningen , 9747 AG , The Netherlands. FAU - Blah, Patrick J AU - Blah PJ AD - Zernike Institute for Advanced Materials , University of Groningen , Groningen , 9747 AG , The Netherlands. FAU - van Wees, Bart J AU - van Wees BJ AD - Zernike Institute for Advanced Materials , University of Groningen , Groningen , 9747 AG , The Netherlands. LA - eng PT - Journal Article DEP - 20190827 PL - United States TA - Nano Lett JT - Nano letters JID - 101088070 SB - IM PMC - PMC6746057 OTO - NOTNLM OT - Rashba spin-orbit coupling OT - Rashba-Edelstein effect OT - proximity effect OT - spin Hall effect OT - valley-Zeeman COIS- The authors declare no competing financial interest. EDAT- 2019/08/14 06:00 MHDA- 2019/08/14 06:01 PMCR- 2019/09/16 CRDT- 2019/08/14 06:00 PHST- 2019/08/14 06:00 [pubmed] PHST- 2019/08/14 06:01 [medline] PHST- 2019/08/14 06:00 [entrez] PHST- 2019/09/16 00:00 [pmc-release] AID - 10.1021/acs.nanolett.9b01611 [doi] PST - ppublish SO - Nano Lett. 2019 Sep 11;19(9):5959-5966. doi: 10.1021/acs.nanolett.9b01611. Epub 2019 Aug 27.