PMID- 31859416
OWN - NLM
STAT- PubMed-not-MEDLINE
LR  - 20200304
IS  - 1613-6829 (Electronic)
IS  - 1613-6810 (Linking)
VI  - 16
IP  - 3
DP  - 2020 Jan
TI  - Direct Growth of Perovskite Crystals on Metallic Electrodes for High-Performance 
      Electronic and Optoelectronic Devices.
PG  - e1906185
LID - 10.1002/smll.201906185 [doi]
AB  - Metal halide perovskite has attracted enhanced interest for its diverse 
      electronic and optoelectronic applications. However, the fabrication of micro- or 
      nanoscale crystalline perovskite functional devices remains a great challenge due 
      to the fragility, solvent, and heat sensitivity of perovskite crystals. Here, a 
      strategy is proposed to fabricate electronic and optoelectronic devices by 
      directly growing perovskite crystals on microscale metallic structures in liquid 
      phase. The well-contacted perovskite/metal interfaces ensure these 
      heterostructures serve as high-performance field effect transistors (FETs) and 
      excellent photodetector devices. When serving as an FET, the on/off ratio is as 
      large as 10(6) and the mobility reaches up to  approximately 2.3 cm(2) V(-1) s(-1) . A 
      photodetector is displayed with high photoconductive switching ratio of  approximately 10(6) 
      and short response time of  approximately 4 ms. Furthermore, the photoconductive response is 
      proved to be band-bending-assisted separation of photoexcited carriers at the 
      Schottky barrier of the silver and p-type perovskites.
CI  - (c) 2019 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
FAU - Liu, Jia
AU  - Liu J
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
FAU - Liu, Fengjing
AU  - Liu F
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
AD  - CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS 
      Center for Excellence in Nanoscience, National Centre for Nanoscience and 
      Technology, Beijing, 100190, China.
FAU - Liu, Haining
AU  - Liu H
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
AD  - CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS 
      Center for Excellence in Nanoscience, National Centre for Nanoscience and 
      Technology, Beijing, 100190, China.
FAU - Hou, Rui
AU  - Hou R
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
AD  - State Key Laboratory of Superlattice and Microstructure, Institute of 
      Semiconductors, Chinese Academy of Science, Beijing, 100083, China.
FAU - Yue, Junyi
AU  - Yue J
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
FAU - Cai, Jinzhong
AU  - Cai J
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
FAU - Peng, Zhisheng
AU  - Peng Z
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
FAU - Impundu, Julienne
AU  - Impundu J
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
AD  - School of Nanoscience and Technology, University of Chinese Academy of Sciences, 
      Beijing, 100049, China.
FAU - Xie, Liming
AU  - Xie L
AD  - CAS Key Laboratory of Standardization and Measurement for Nanotechnology, CAS 
      Center for Excellence in Nanoscience, National Centre for Nanoscience and 
      Technology, Beijing, 100190, China.
FAU - Li, Yong Jun
AU  - Li YJ
AUID- ORCID: 0000-0001-6645-5209
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
FAU - Sun, Lianfeng
AU  - Sun L
AD  - CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, CAS Centre for 
      Excellence in Nanoscience, National Centre for Nanoscience and Technology, 
      Beijing, 100190, China.
LA  - eng
GR  - 21973021/National Natural Science Foundation of China/
GR  - 21603241/National Natural Science Foundation of China/
GR  - 11874129/National Natural Science Foundation of China/
GR  - 2018YFA0208403/Chinese Ministry of Science and Technology/
GR  - 2016YFA0200403/Chinese Ministry of Science and Technology/
GR  - Baotou Rare Earth Research and Development Centre/
GR  - GZR 2018001/Chinese Academy of Sciences/
PT  - Journal Article
DEP - 20191220
PL  - Germany
TA  - Small
JT  - Small (Weinheim an der Bergstrasse, Germany)
JID - 101235338
SB  - IM
OTO - NOTNLM
OT  - field effect transistors
OT  - heterostructures
OT  - metal halide perovskites
OT  - photodetectors
EDAT- 2019/12/21 06:00
MHDA- 2019/12/21 06:01
CRDT- 2019/12/21 06:00
PHST- 2019/10/28 00:00 [received]
PHST- 2019/11/26 00:00 [revised]
PHST- 2019/12/21 06:00 [pubmed]
PHST- 2019/12/21 06:01 [medline]
PHST- 2019/12/21 06:00 [entrez]
AID - 10.1002/smll.201906185 [doi]
PST - ppublish
SO  - Small. 2020 Jan;16(3):e1906185. doi: 10.1002/smll.201906185. Epub 2019 Dec 20.