PMID- 31941637 OWN - NLM STAT- MEDLINE DCOM- 20200225 LR - 20220531 IS - 1095-8630 (Electronic) IS - 0301-4797 (Linking) VI - 260 DP - 2020 Apr 15 TI - Remediation of persistent organic pollutants in aqueous systems by electrochemical activation of persulfates: A review. PG - 110125 LID - S0301-4797(20)30063-3 [pii] LID - 10.1016/j.jenvman.2020.110125 [doi] AB - Sulfate-radical-based advanced oxidation processes (SR-AOPs) have been widely applied in environmental remediation during the past decade, especially in the degradation of refractory organic contaminants. The electrochemical method, which is considered as one of the most efficient ways to generate sulfate radical, has been extensively investigated for the activation of persulfate recently. This work presented a thorough assessment towards the performance of electrochemically activated persulfate for the removal of persistent organic pollutants (POPs) in aqueous systems. The mechanism and superiority of electrochemically activated persulfates were revealed accordingly. Some major factors (e.g., electrode material, pH, current density, and persulfate concentration) influencing the electrochemical activation of persulfates to remove POPs were also discussed. Considering the increasing quantity of publications on this subject, it is significant to broader guidelines such as the efficiency for practical application, quantization of organic by-products, and cost-effectiveness of the electrochemical method to optimize active persulfate in the water treatment processes. CI - Copyright (c) 2020 Elsevier Ltd. All rights reserved. FAU - Zhi, Dan AU - Zhi D AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. FAU - Lin, Yinghui AU - Lin Y AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. FAU - Jiang, Li AU - Jiang L AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. FAU - Zhou, Yaoyu AU - Zhou Y AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. Electronic address: zhouyy@hunau.edu.cn. FAU - Huang, Anqi AU - Huang A AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. FAU - Yang, Jian AU - Yang J AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. FAU - Luo, Lin AU - Luo L AD - College of Resources and Environment, Hunan Agricultural University, Changsha, 410128, PR China. LA - eng PT - Journal Article PT - Review DEP - 20200117 PL - England TA - J Environ Manage JT - Journal of environmental management JID - 0401664 RN - 0 (Environmental Pollutants) RN - 0 (Sulfates) RN - 0 (Water Pollutants, Chemical) RN - 059QF0KO0R (Water) SB - IM MH - *Environmental Pollutants MH - *Environmental Restoration and Remediation MH - Oxidation-Reduction MH - Sulfates MH - Water MH - *Water Pollutants, Chemical MH - *Water Purification OTO - NOTNLM OT - Electrochemical activation OT - Environmental remediation OT - Influencing factors OT - Mechanisms OT - Persulfates OT - Practical application COIS- Declaration of competing interest There is no conflict of interest associated with this work. EDAT- 2020/01/17 06:00 MHDA- 2020/02/26 06:00 CRDT- 2020/01/17 06:00 PHST- 2019/10/25 00:00 [received] PHST- 2020/01/02 00:00 [revised] PHST- 2020/01/10 00:00 [accepted] PHST- 2020/01/17 06:00 [pubmed] PHST- 2020/02/26 06:00 [medline] PHST- 2020/01/17 06:00 [entrez] AID - S0301-4797(20)30063-3 [pii] AID - 10.1016/j.jenvman.2020.110125 [doi] PST - ppublish SO - J Environ Manage. 2020 Apr 15;260:110125. doi: 10.1016/j.jenvman.2020.110125. Epub 2020 Jan 17.