PMID- 32115783 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20200930 IS - 1521-4095 (Electronic) IS - 0935-9648 (Linking) VI - 32 IP - 16 DP - 2020 Apr TI - Metasurface-Enabled Generation of Circularly Polarized Single Photons. PG - e1907832 LID - 10.1002/adma.201907832 [doi] AB - Single photons carrying spin angular momentum (SAM), i.e., circularly polarized single photons generated typically by subjecting a quantum emitter (QE) to a strong magnetic field at low temperatures, are at the core of chiral quantum optics enabling nonreciprocal single-photon configurations and deterministic spin-photon interfaces. Here, a conceptually new approach to the room-temperature generation of SAM-coded single photons (SSPs) is described, which entails QE nonradiative coupling to surface plasmons being transformed, by interacting with an optical metasurface, into a collimated stream of SSPs with the designed handedness. Design, fabrication, and characterization of SSP sources, consisting of dielectric circular nanoridges with azimuthally varying widths deterministically fabricated on a dielectric-protected silver film around a nanodiamond containing a nitrogen-vacancy center, are reported. With properly engineered phases of QE-originated fields scattered by nanoridges, the outcoupled photons are characterized by a well-defined SAM (with the chirality >0.8) and high directionality (collection efficiency up to 92%). CI - (c) 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. FAU - Kan, Yinhui AU - Kan Y AD - Institute of Engineering Thermophysics, Shanghai Jiao Tong University, Shanghai, 200240, China. AD - Center for Nano Optics, University of Southern Denmark, DK-5230, Odense M, Denmark. FAU - Andersen, Sebastian K H AU - Andersen SKH AD - Center for Nano Optics, University of Southern Denmark, DK-5230, Odense M, Denmark. FAU - Ding, Fei AU - Ding F AD - Center for Nano Optics, University of Southern Denmark, DK-5230, Odense M, Denmark. FAU - Kumar, Shailesh AU - Kumar S AD - Center for Nano Optics, University of Southern Denmark, DK-5230, Odense M, Denmark. FAU - Zhao, Changying AU - Zhao C AD - Institute of Engineering Thermophysics, Shanghai Jiao Tong University, Shanghai, 200240, China. FAU - Bozhevolnyi, Sergey I AU - Bozhevolnyi SI AUID- ORCID: 0000-0002-0393-4859 AD - Center for Nano Optics, University of Southern Denmark, DK-5230, Odense M, Denmark. LA - eng GR - Villum Kann Rasmussen Foundation/ GR - 00022988/Villum Fonden/ GR - 51636004/National Natural Science Foundation of China/ GR - 201806230179/China Scholarship Council/ GR - 341054/ERC_/European Research Council/International PT - Journal Article DEP - 20200301 PL - Germany TA - Adv Mater JT - Advanced materials (Deerfield Beach, Fla.) JID - 9885358 SB - IM OTO - NOTNLM OT - circular polarization OT - metasurfaces OT - quantum emitters OT - single photons OT - surface plasmon polaritons EDAT- 2020/03/03 06:00 MHDA- 2020/03/03 06:01 CRDT- 2020/03/03 06:00 PHST- 2019/11/28 00:00 [received] PHST- 2020/01/28 00:00 [revised] PHST- 2020/03/03 06:00 [pubmed] PHST- 2020/03/03 06:01 [medline] PHST- 2020/03/03 06:00 [entrez] AID - 10.1002/adma.201907832 [doi] PST - ppublish SO - Adv Mater. 2020 Apr;32(16):e1907832. doi: 10.1002/adma.201907832. Epub 2020 Mar 1.