PMID- 32247975 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20200512 LR - 20200518 IS - 1879-1026 (Electronic) IS - 0048-9697 (Linking) VI - 724 DP - 2020 Jul 1 TI - Influence of TiO(2)-based photocatalytic coating road on traffic-related NO(x) pollutants in urban street canyon by CFD modeling. PG - 138059 LID - S0048-9697(20)31572-2 [pii] LID - 10.1016/j.scitotenv.2020.138059 [doi] AB - The use of titanium dioxide (TiO(2)) photocatalytic nanoparticles as road coating to trap and decompose air pollutants provides a promising technology to mitigate the harmful effects of vehicle emissions. However, there are few studies on computational fluid dynamics (CFD) simulations of the effect of NOx photocatalytic oxidation in street canyon with TiO(2) nanoparticles as pavement coating. This study develop a CFD model with photocatalytic oxidation (PCO) reaction implemented for numerical simulation of NO(x) abatement in an urban street canyon with TiO(2) coating, considering the effects of relative humidity (RH) (10-90%), and irradiance (10-40W ⋅ m(-2)). Results show that TiO(2) coating road can effectively reduce nitrogen oxide (NO(x)) concentration in the street canyon. The average nitric oxide (NO) and nitrogen dioxide (NO(2)) concentrations in street canyon with TiO(2) coating road were reduced by 3.70% and 4.31%, respectively, comparing with street canyon without TiO(2) coating. The irradiance and relative humidity had great effect on PCO reaction in street canyon with TiO(2) coating road. When the irradiance increased from 10W ⋅ m(-2) to 40W ⋅ m(-2)(,) average NO conversion rose from 1.35% to 3.70%, and average NO(2) conversion rose from 2.43% to 4.31%. The average conversion of NO and NO(2) decreased from 5.11% to 2.54% and from 5.60% to 3.25%, respectively, when the relative humidity is varied from 10% to 90%. Results are useful to transport planners and road engineers who need to reduce NOx concentrations in urban streets travelled by fossil fuel-powered vehicles. Method of the study can be considered by future research faced with different pavement construction and traffic environment. CI - Copyright (c) 2020 Elsevier B.V. All rights reserved. FAU - Xie, Xiaomin AU - Xie X AD - Key Laboratory for Power machinery and Engineering of M. O. E., Shanghai Jiao Tong University, No. 800, Dongchuan Road, 200240 Shanghai, PR China. Electronic address: xiexiaomin@sjtu.edu.cn. FAU - Hao, Chenrui AU - Hao C AD - Key Laboratory for Power machinery and Engineering of M. O. E., Shanghai Jiao Tong University, No. 800, Dongchuan Road, 200240 Shanghai, PR China. FAU - Huang, Yue AU - Huang Y AD - Institute for Transport Studies, University of Leeds, 34-40 University Road, Leeds LS2 9JT, UK. FAU - Huang, Zhen AU - Huang Z AD - Key Laboratory for Power machinery and Engineering of M. O. E., Shanghai Jiao Tong University, No. 800, Dongchuan Road, 200240 Shanghai, PR China. LA - eng PT - Journal Article DEP - 20200319 PL - Netherlands TA - Sci Total Environ JT - The Science of the total environment JID - 0330500 SB - IM OTO - NOTNLM OT - Computational fluid dynamics (CFD) simulation OT - NO(x) concentration OT - Photocatalytic oxidation (PCO) OT - Street canyon OT - TiO(2) coating road COIS- Declaration of competing interest The authors declare no competing financial interests. EDAT- 2020/04/06 06:00 MHDA- 2020/04/06 06:01 CRDT- 2020/04/06 06:00 PHST- 2020/01/02 00:00 [received] PHST- 2020/03/02 00:00 [revised] PHST- 2020/03/18 00:00 [accepted] PHST- 2020/04/06 06:00 [pubmed] PHST- 2020/04/06 06:01 [medline] PHST- 2020/04/06 06:00 [entrez] AID - S0048-9697(20)31572-2 [pii] AID - 10.1016/j.scitotenv.2020.138059 [doi] PST - ppublish SO - Sci Total Environ. 2020 Jul 1;724:138059. doi: 10.1016/j.scitotenv.2020.138059. Epub 2020 Mar 19.