PMID- 32315799 OWN - NLM STAT- MEDLINE DCOM- 20210514 LR - 20210514 IS - 1873-3336 (Electronic) IS - 0304-3894 (Linking) VI - 395 DP - 2020 Aug 5 TI - Interface engineering of zeolite imidazolate framework-8 on two-dimensional Al-metal-organic framework nanoplates enhancing performance for simultaneous capture and sensing tetracyclines. PG - 122615 LID - S0304-3894(20)30604-X [pii] LID - 10.1016/j.jhazmat.2020.122615 [doi] AB - The increasing misgivings of environmental pollution derived from antibiotic residues make it imperative to explore a bifunctional platform for synchronous monitoring and removal of antibiotics. Herein, zeolite imidazolate framework-8 (ZIF-8) is anchored on two-dimensional (2D) amino-functionalized Al-metal organic framework (NH(2)-MIL-53(Al)) nanoplates to construct a dual metal-organic frameworks smart platform (ZIF-8/NH(2)-MIL-53(Al)) for simultaneous capture and fluorescence sensing of tetracyclines (TCs). ZIF-8 nanoparticles anchored on 2D nanoplates having a smaller size and a larger specific surface area boost the adsorption capabilities (561, 533, 526 and 578 mg g(-1) for doxycycline (DOX), tetracycline (TET), oxytetracycline (OTC) and chlortetracycline (CTC), respectively). Notably, the pyridine N of ZIF-8 cooperated with the abundant NH(2) on the surface of NH(2)-MIL-53(Al) exhibits high affinity toward TCs, remarkably enhancing the sensitivity by facilitating the photo-induced electron transfer and the inner-filter effect. The LODs (1.2 mug L(-1) for TET, DOX, OTC and 2.2 mug L(-1) for CTC, respectively) are at least 10-fold lower than those of NH(2)-MIL-53(Al) and are comparable or superior to those of reported sensors. The dual metal-organic frameworks smart platform presents satisfactory reliabilities and accuracies for detecting TCs in real samples, which anticipates new routes to develop integrated systems for simultaneous capture and detection of organic pollutants. CI - Copyright (c) 2020 Elsevier B.V. All rights reserved. FAU - Li, Chunhua AU - Li C AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Zhang, Xiaoshuo AU - Zhang X AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Wen, Simin AU - Wen S AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Xiang, Rui AU - Xiang R AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Han, Yong AU - Han Y AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Tang, Wenzhi AU - Tang W AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China. FAU - Yue, Tianli AU - Yue T AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China; Laboratory of Quality & Safety Risk Assessment for Agro-products (Yangling), Ministry of Agriculture, Yangling, 712100, Shaanxi, China. FAU - Li, Zhonghong AU - Li Z AD - College of Food Science and Engineering, Northwest A&F University, Yangling, 712100, Shaanxi, China; Laboratory of Quality & Safety Risk Assessment for Agro-products (Yangling), Ministry of Agriculture, Yangling, 712100, Shaanxi, China. Electronic address: steveli@nwsuaf.edu.cn. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20200407 PL - Netherlands TA - J Hazard Mater JT - Journal of hazardous materials JID - 9422688 RN - 0 (Anti-Bacterial Agents) RN - 0 (Metal-Organic Frameworks) RN - 0 (Tetracyclines) RN - 1318-02-1 (Zeolites) RN - X20I9EN955 (Oxytetracycline) SB - IM MH - Anti-Bacterial Agents MH - *Metal-Organic Frameworks MH - *Oxytetracycline MH - Tetracyclines MH - *Zeolites OTO - NOTNLM OT - Antibiotic residues OT - MOF-on-MOF OT - Metal-organic framework OT - Simultaneous adsorption and detection OT - Water remediation EDAT- 2020/04/22 06:00 MHDA- 2021/05/15 06:00 CRDT- 2020/04/22 06:00 PHST- 2019/11/19 00:00 [received] PHST- 2020/03/28 00:00 [revised] PHST- 2020/03/28 00:00 [accepted] PHST- 2020/04/22 06:00 [pubmed] PHST- 2021/05/15 06:00 [medline] PHST- 2020/04/22 06:00 [entrez] AID - S0304-3894(20)30604-X [pii] AID - 10.1016/j.jhazmat.2020.122615 [doi] PST - ppublish SO - J Hazard Mater. 2020 Aug 5;395:122615. doi: 10.1016/j.jhazmat.2020.122615. Epub 2020 Apr 7.