PMID- 32584582 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20200930 IS - 1530-6992 (Electronic) IS - 1530-6984 (Linking) VI - 20 IP - 8 DP - 2020 Aug 12 TI - Control of Spin-Orbit Torques by Interface Engineering in Topological Insulator Heterostructures. PG - 5893-5899 LID - 10.1021/acs.nanolett.0c01850 [doi] AB - (Bi(1-x)Sb(x))(2)Te(3) topological insulators (TIs) are gathering increasing attention owing to their large charge-to-spin conversion efficiency and the ensuing spin-orbit torques (SOTs) that can be used to manipulate the magnetization of a ferromagnet (FM). The origin of the torques, however, remains elusive, while the implications of hybridized states and the strong material intermixing at the TI/FM interface are essentially unexplored. By combining interface chemical analysis and spin-transfer ferromagnetic resonance (ST-FMR) measurements, we demonstrate that intermixing plays a critical role in the generation of SOTs. By inserting a suitable normal metal spacer, material intermixing is reduced and the TI properties at the interface are largely improved, resulting in strong variations in the nature of the SOTs. A dramatic enhancement of a field-like torque, opposing and surpassing the Oersted-field torque, is observed, which can be attributed to the non-equilibrium spin density in Rashba-split surface bands and to the suppression of spin memory loss. These phenomena can play a relevant role at other interfaces, such as those comprising transition metal dichalcogenides. FAU - Bonell, Frederic AU - Bonell F AUID- ORCID: 0000-0001-7296-0404 AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. FAU - Goto, Minori AU - Goto M AD - Graduate School of Engineering Science and Center for Spintronics Research Network (CSRN), Osaka University, Toyonaka, Osaka 560-8531, Japan. FAU - Sauthier, Guillaume AU - Sauthier G AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. FAU - Sierra, Juan F AU - Sierra JF AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. FAU - Figueroa, Adriana I AU - Figueroa AI AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. FAU - Costache, Marius V AU - Costache MV AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. FAU - Miwa, Shinji AU - Miwa S AUID- ORCID: 0000-0001-9131-6753 AD - Graduate School of Engineering Science and Center for Spintronics Research Network (CSRN), Osaka University, Toyonaka, Osaka 560-8531, Japan. FAU - Suzuki, Yoshishige AU - Suzuki Y AD - Graduate School of Engineering Science and Center for Spintronics Research Network (CSRN), Osaka University, Toyonaka, Osaka 560-8531, Japan. FAU - Valenzuela, Sergio O AU - Valenzuela SO AUID- ORCID: 0000-0002-4632-8891 AD - Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC, and The Barcelona Institute of Science and Technology (BIST), Campus UAB, Bellaterra, 08193 Barcelona, Spain. AD - Institucio Catalana de Recerca i Estudis Avancats (ICREA), 08070 Barcelona, Spain. LA - eng PT - Journal Article DEP - 20200702 PL - United States TA - Nano Lett JT - Nano letters JID - 101088070 SB - IM OTO - NOTNLM OT - Topological insulator OT - spin memory loss OT - spin-torque ferromagnetic resonance OT - spin-orbit torque EDAT- 2020/06/26 06:00 MHDA- 2020/06/26 06:01 CRDT- 2020/06/26 06:00 PHST- 2020/06/26 06:00 [pubmed] PHST- 2020/06/26 06:01 [medline] PHST- 2020/06/26 06:00 [entrez] AID - 10.1021/acs.nanolett.0c01850 [doi] PST - ppublish SO - Nano Lett. 2020 Aug 12;20(8):5893-5899. doi: 10.1021/acs.nanolett.0c01850. Epub 2020 Jul 2.