PMID- 33144015 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20210526 LR - 20210526 IS - 1873-3336 (Electronic) IS - 0304-3894 (Linking) VI - 407 DP - 2021 Apr 5 TI - Spatial distribution, deposition flux, and environmental impact of typical persistent organic pollutants in surficial sediments in the Eastern China Marginal Seas (ECMSs). PG - 124343 LID - S0304-3894(20)32333-5 [pii] LID - 10.1016/j.jhazmat.2020.124343 [doi] AB - High emissions of synthetic compounds are damaging the marine environment and threatening human health. This study represents the first extensive and comprehensive analysis of three typical persistent organic pollutants (POPs), i.e., organochlorine pesticides (n = 228), perfluoroalkyl substances (n = 202), and short-chain chlorinated paraffins (n = 162), using a highly resolved spatial dataset. The results revealed the complex distribution of POPs in the Eastern China Marginal Seas (ECMSs). POPs in the surface sediments of the ECMSs showed spatial heterogeneity, with high levels observed mainly in areas with fine-grained sediments (e.g., the Yellow River and Changjiang River estuaries and the central south Yellow Sea). Strong positive correlations were identified between POP concentration and sediment grain size/components/longitude/latitude in the ECMSs, suggesting that POP distribution was significantly influenced by river input and regional hydrodynamics. The annual deposition fluxes of POPs in the ECMSs were also calculated and high values were recorded in the Yellow River Estuary and East China Sea. Human-induced changes in the catchments could affect the fate of POPs in the ECMSs and other river-dominated marginal seas worldwide. Our findings highlight concerns regarding local aquaculture and provide a basis for government decision-making. We also suggest the need for increased attention to be paid to the effects of marine organic pollution on aquaculture on a global scale. CI - Copyright (c) 2020 Elsevier B.V. All rights reserved. FAU - Hao, Zhe AU - Hao Z AD - Key Laboratory of Engineering Oceanography, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou, China; School of Geographic and Oceanographic Sciences, Ministry of Education Key Laboratory for Coast and Island Development, Nanjing University, Nanjing 210093, China; Collaborative Innovation Center of South China Sea Studies, Nanjing University, Nanjing 210093, China. FAU - Xu, Hengtao AU - Xu H AD - Key Laboratory of Engineering Oceanography, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou, China. Electronic address: xuht@sio.org.cn. FAU - Feng, Ziyue AU - Feng Z AD - School of Geographic and Oceanographic Sciences, Ministry of Education Key Laboratory for Coast and Island Development, Nanjing University, Nanjing 210093, China. FAU - Zhang, Chuchu AU - Zhang C AD - School of Geographic and Oceanographic Sciences, Ministry of Education Key Laboratory for Coast and Island Development, Nanjing University, Nanjing 210093, China. FAU - Zhou, Xin AU - Zhou X AD - First Institute of Oceanography, Ministry of Natural Resources, Qingdao, China. FAU - Wang, Zhifu AU - Wang Z AD - Key Laboratory of Engineering Oceanography, Second Institute of Oceanography, Ministry of Natural Resources, Hangzhou, China. FAU - Zheng, Jiaheng AU - Zheng J AD - First Institute of Oceanography, Ministry of Natural Resources, Qingdao, China. FAU - Zou, Xinqing AU - Zou X AD - School of Geographic and Oceanographic Sciences, Ministry of Education Key Laboratory for Coast and Island Development, Nanjing University, Nanjing 210093, China; Collaborative Innovation Center of South China Sea Studies, Nanjing University, Nanjing 210093, China. Electronic address: zouxq@nju.edu.cn. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20201021 PL - Netherlands TA - J Hazard Mater JT - Journal of hazardous materials JID - 9422688 SB - IM OTO - NOTNLM OT - Deposition flux OT - Depositional process OT - ECMSs OT - Grain size OT - POPs EDAT- 2020/11/05 06:00 MHDA- 2020/11/05 06:01 CRDT- 2020/11/04 05:34 PHST- 2020/05/20 00:00 [received] PHST- 2020/10/14 00:00 [revised] PHST- 2020/10/17 00:00 [accepted] PHST- 2020/11/05 06:00 [pubmed] PHST- 2020/11/05 06:01 [medline] PHST- 2020/11/04 05:34 [entrez] AID - S0304-3894(20)32333-5 [pii] AID - 10.1016/j.jhazmat.2020.124343 [doi] PST - ppublish SO - J Hazard Mater. 2021 Apr 5;407:124343. doi: 10.1016/j.jhazmat.2020.124343. Epub 2020 Oct 21.