PMID- 34144550 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20210706 IS - 1361-6528 (Electronic) IS - 0957-4484 (Linking) VI - 32 IP - 38 DP - 2021 Jul 2 TI - Facile and effective repair of Pt/Nafion IPMC actuator by dip-coating of PVP@AgNPs. LID - 10.1088/1361-6528/ac0cae [doi] AB - Ionic polymer metal composite (IPMC) always takes big risks of electrode cracking and peeling, which lead to energy wasting, waterloss, and uneven electric field distribution, thus hamper its commercial applications. To address this issue, we propose a facile and effective technique to repair the electrode fatigue by coating polyvinylpyrrolidone (PVP) encapsulated Ag nanoparticles (PVP@AgNPs) on the long-term used IPMC surface. To improve the electrochemical stability, the silver nanoparticles (Ag NPs) with a diameter of approximately 34 nm are encapsulated by a 1.3 nm thick PVP film, thus forming a shell-core structure to resist corrosion from the electrolyte solution. Physiochemical investigations reveal that, PVP@AgNPs closely attach to the interior and exterior surfaces of the original Pt nanograin electrode, thus refreshing its electronic conductivity; the repaired IPMC actuator exhibits better electromechanical properties compared to its precursor actuator: 7.62 folds in displacement output, 9.38 folds in force output, and 9.73 folds in stable working time. CI - (c) 2021 IOP Publishing Ltd. FAU - Wang, Fang AU - Wang F AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. FAU - Zhang, Xiaodie AU - Zhang X AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. FAU - Ma, Li AU - Ma L AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. FAU - Zhang, Zhiqiang AU - Zhang Z AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. FAU - Han, Lifeng AU - Han L AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. FAU - Zeng, Chao AU - Zeng C AD - College of Information Science and Engineering, Henan University of Technology, Zhengzhou 450001, People's Republic of China. FAU - Shi, Bo AU - Shi B AD - College of Energy and Power Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, People's Republic of China. FAU - Guo, Dongjie AU - Guo D AUID- ORCID: 0000-0002-9426-7544 AD - State Laboratory of Surface & Interface, Zhengzhou University of Light Industry, Zhengzhou 450002, People's Republic of China. LA - eng PT - Journal Article DEP - 20210702 PL - England TA - Nanotechnology JT - Nanotechnology JID - 101241272 SB - IM OTO - NOTNLM OT - electroactive polymer (EAP) OT - electrode fatigue OT - electromechanical response OT - granular damming effect OT - ionic polymer metal composite (IPMC) EDAT- 2021/06/19 06:00 MHDA- 2021/06/19 06:01 CRDT- 2021/06/18 20:30 PHST- 2021/05/23 00:00 [received] PHST- 2021/06/18 00:00 [accepted] PHST- 2021/06/19 06:00 [pubmed] PHST- 2021/06/19 06:01 [medline] PHST- 2021/06/18 20:30 [entrez] AID - 10.1088/1361-6528/ac0cae [doi] PST - epublish SO - Nanotechnology. 2021 Jul 2;32(38). doi: 10.1088/1361-6528/ac0cae.