PMID- 34569100 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20211201 IS - 1521-4095 (Electronic) IS - 0935-9648 (Linking) VI - 33 IP - 48 DP - 2021 Dec TI - Highly Sensitive Capacitive Pressure Sensors over a Wide Pressure Range Enabled by the Hybrid Responses of a Highly Porous Nanocomposite. PG - e2103320 LID - 10.1002/adma.202103320 [doi] AB - Past research aimed at increasing the sensitivity of capacitive pressure sensors has mostly focused on developing dielectric layers with surface/porous structures or higher dielectric constants. However, such strategies have only been effective in improving sensitivities at low pressure ranges (e.g., up to 3 kPa). To overcome this well-known obstacle, herein, a flexible hybrid-response pressure sensor (HRPS) composed of an electrically conductive porous nanocomposite (PNC) laminated with an ultrathin dielectric layer is devised. Using a nickel foam template, the PNC is fabricated with carbon nanotubes (CNTs)-doped Ecoflex to be 86% porous and electrically conductive. The PNC exhibits hybrid piezoresistive and piezocapacitive responses, resulting in significantly enhanced sensitivities (i.e., more than 400%) over wide pressure ranges, from 3.13 kPa(-1) within 0-1 kPa to 0.43 kPa(-1) within 30-50 kPa. The effect of the hybrid responses is differentiated from the effect of porosity or high dielectric constants by comparing the HRPS with its purely piezocapacitive counterparts. Fundamental understanding of the HRPS and the prediction of optimal CNT doping are achieved through simplified analytical models. The HRPS is able to measure pressures from as subtle as the temporal arterial pulse to as large as footsteps. CI - (c) 2021 Wiley-VCH GmbH. FAU - Ha, Kyoung-Ho AU - Ha KH AD - Department of Mechanical Engineering, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Zhang, Weiyi AU - Zhang W AD - Department of Aerospace Engineering and Engineering Mechanics, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Jang, Hongwoo AU - Jang H AD - Texas Material Institute, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Kang, Seungmin AU - Kang S AD - Department of Biomedical Engineering, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Wang, Liu AU - Wang L AD - Department of Aerospace Engineering and Engineering Mechanics, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Tan, Philip AU - Tan P AD - Department of Electrical and Computer Engineering, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Hwang, Hochul AU - Hwang H AD - Department of Aerospace Engineering and Engineering Mechanics, University of Texas at Austin, Austin, TX, 78712, USA. FAU - Lu, Nanshu AU - Lu N AUID- ORCID: 0000-0002-3595-3851 AD - Department of Aerospace Engineering and Engineering Mechanics, Department of Electrical and Computer Engineering, Department of Mechanical Engineering, Department of Biomedical Engineering, Texas Materials Institute, University of Texas at Austin, Austin, TX, 78712, USA. LA - eng GR - N00014-20-1-2112/Office of Naval Research/ GR - N00014-18-1-2323/Office of Naval Research/ GR - W911NF-19-2-0333/Army Research Office/ PT - Journal Article DEP - 20210927 PL - Germany TA - Adv Mater JT - Advanced materials (Deerfield Beach, Fla.) JID - 9885358 SB - IM OTO - NOTNLM OT - conductive foams OT - e-skins OT - flexible electronics OT - porous nanocomposites OT - pressure sensors OT - pulse waveforms EDAT- 2021/09/28 06:00 MHDA- 2021/09/28 06:01 CRDT- 2021/09/27 06:35 PHST- 2021/07/27 00:00 [revised] PHST- 2021/04/30 00:00 [received] PHST- 2021/09/28 06:00 [pubmed] PHST- 2021/09/28 06:01 [medline] PHST- 2021/09/27 06:35 [entrez] AID - 10.1002/adma.202103320 [doi] PST - ppublish SO - Adv Mater. 2021 Dec;33(48):e2103320. doi: 10.1002/adma.202103320. Epub 2021 Sep 27.