PMID- 34640080 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20211016 IS - 1996-1944 (Print) IS - 1996-1944 (Electronic) IS - 1996-1944 (Linking) VI - 14 IP - 19 DP - 2021 Sep 29 TI - Photocatalytic Inactivation of Salmonella typhimurium by Floating Carbon-Doped TiO(2) Photocatalyst. LID - 10.3390/ma14195681 [doi] LID - 5681 AB - Photocatalysis application is considered as one of the most highly promising techniques for the reduction in wastewater pollution. However, the majority of highly efficient photocatalyst materials are obtained as fine powders, and this causes a lot of photocatalyst handling and reusability issues. The concept of the floating catalyst proposes the immobilization of a photocatalytic (nano)material on relatively large floating substrates and is considered as an encouraging way to overcome some of the most challenging photocatalysis issues. The purpose of this study is to examine floating photocatalyst application for Salmonella typhimurium bacteria inactivation in polluted water. More specifically, high-density polyethylene (HDPE) beads were used as a photocatalyst support for the immobilization of carbon-doped TiO(2) films forming floating photocatalyst structures. Carbon-doped TiO(2) films in both amorphous and anatase forms were deposited on HDPE beads using the low-temperature magnetron sputtering technique. Bacteria inactivation, together with cycling experiments, revealed promising results by decomposing more than 95% of Salmonella typhimurium bacteria in five consecutive treatment cycles. Additionally, a thorough analysis of the deposited carbon-doped TiO(2) film was performed including morphology, elemental composition and mapping, structure, and depth profiling. The results demonstrate that the proposed method is a suitable technique for the formation of high-quality photocatalytic active films on thermal-sensitive substrates. FAU - Varnagiris, Sarunas AU - Varnagiris S AD - Center for Hydrogen Energy Technologies, Lithuanian Energy Institute, 3 Breslaujos, 44403 Kaunas, Lithuania. FAU - Urbonavicius, Marius AU - Urbonavicius M AUID- ORCID: 0000-0001-7538-9733 AD - Center for Hydrogen Energy Technologies, Lithuanian Energy Institute, 3 Breslaujos, 44403 Kaunas, Lithuania. FAU - Sakalauskaite, Sandra AU - Sakalauskaite S AD - Department of Biochemistry, Faculty of Natural Sciences, Vytautas Magnus University, 8 Vileikos, 44404 Kaunas, Lithuania. FAU - Demikyte, Emilija AU - Demikyte E AUID- ORCID: 0000-0002-5123-2683 AD - Department of Biochemistry, Faculty of Natural Sciences, Vytautas Magnus University, 8 Vileikos, 44404 Kaunas, Lithuania. FAU - Tuckute, Simona AU - Tuckute S AD - Center for Hydrogen Energy Technologies, Lithuanian Energy Institute, 3 Breslaujos, 44403 Kaunas, Lithuania. FAU - Lelis, Martynas AU - Lelis M AD - Center for Hydrogen Energy Technologies, Lithuanian Energy Institute, 3 Breslaujos, 44403 Kaunas, Lithuania. LA - eng GR - 09.3.3-LMT-K-712-01-0175/Lietuvos Mokslu Akademija/ PT - Journal Article DEP - 20210929 PL - Switzerland TA - Materials (Basel) JT - Materials (Basel, Switzerland) JID - 101555929 PMC - PMC8510230 OTO - NOTNLM OT - Salmonella typhimurium OT - carbon-doped TiO2 OT - floating photocatalyst OT - magnetron sputtering OT - thin films COIS- The authors declare no conflict of interest. EDAT- 2021/10/14 06:00 MHDA- 2021/10/14 06:01 PMCR- 2021/09/29 CRDT- 2021/10/13 01:09 PHST- 2021/08/24 00:00 [received] PHST- 2021/09/17 00:00 [revised] PHST- 2021/09/25 00:00 [accepted] PHST- 2021/10/13 01:09 [entrez] PHST- 2021/10/14 06:00 [pubmed] PHST- 2021/10/14 06:01 [medline] PHST- 2021/09/29 00:00 [pmc-release] AID - ma14195681 [pii] AID - materials-14-05681 [pii] AID - 10.3390/ma14195681 [doi] PST - epublish SO - Materials (Basel). 2021 Sep 29;14(19):5681. doi: 10.3390/ma14195681.