PMID- 34832356 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20211130 IS - 1996-1944 (Print) IS - 1996-1944 (Electronic) IS - 1996-1944 (Linking) VI - 14 IP - 22 DP - 2021 Nov 17 TI - Influence of Potassium-Based Alkaline Electrolyzed Water on Hydration Process and the Properties of Cement-Based Materials with Fly Ash. LID - 10.3390/ma14226956 [doi] LID - 6956 AB - Alkaline electrolyzed water, a kind of clean green water with excellent characteristics such as high activity, strong alkalinity, high ion penetrating ability, electrical charge, and good molecule adsorption, was significant to the resource utilization of industrial fly ash waste. This paper studies highly active potassium-based alkaline electrolyzed water's impact, compared with ordinary water, on the cement hydration process using microstructural methods such as a hydration heat test, differential thermal analysis, X-ray diffraction (XRD) pattern, and Scanning electron microscope (SEM) image analysis. Fly ash cement-based materials were first prepared with alkaline electrolyzed water as the mixing water. The alkaline electrolyzed water's influence on fly ash paste workability and the mechanical properties of fly ash mortar for varying fly ash proportions were ratified. Then alkaline electrolyzed water with the best pH value was selected to prepare fly ash concrete, and its durability was studied. The test results showed that it is feasible to increase the utilization rate of fly ash by using alkaline electrolyzed water. Furthermore, it promoted the process of cement hydration, increased the rate of the hydration reaction, and the promotion effect increased with the increase in pH value of the alkaline electrolyzed water, and also promoted the effective decomposition of the vitreous shell of fly ash to stimulate its early activity. Concurrent tests with ordinary water paste showed that the water requirement for normal consistency and setting time with alkaline electrolyzed water paste were significantly less. Alkaline electrolyzed water also solved the problem related to the low early strength of fly ash mortar. Furthermore, using alkaline electrolyzed water with an optimum pH value of 11.5 to prepare fly ash concrete effectively reduced concrete's carbonation depth and carbonation rate and lessened the chloride ion migration coefficient. FAU - Yu, Zexin AU - Yu Z AUID- ORCID: 0000-0001-8947-2247 AD - School of Architectural Engineering, Qingdao Agricultural University, Qingdao 266109, China. AD - School of Civil Engineering, Qingdao University of Technology, Qingdao 266033, China. FAU - Xie, Zixi AU - Xie Z AD - School of Architectural Engineering, Qingdao Agricultural University, Qingdao 266109, China. FAU - Zhang, Tianyu AU - Zhang T AD - School of Civil Engineering, Qingdao University of Technology, Qingdao 266033, China. FAU - Yue, Gongbing AU - Yue G AD - School of Architectural Engineering, Qingdao Agricultural University, Qingdao 266109, China. FAU - Liu, Haibao AU - Liu H AD - School of Civil Engineering, Qingdao University of Technology, Qingdao 266033, China. FAU - Li, Qiuyi AU - Li Q AD - School of Architectural Engineering, Qingdao Agricultural University, Qingdao 266109, China. FAU - Wang, Liang AU - Wang L AD - School of Architectural Engineering, Qingdao Agricultural University, Qingdao 266109, China. LA - eng GR - 52078261/The National Natural Science Foundation of China/ GR - 51978353/The National Natural Science Foundation of China/ PT - Journal Article DEP - 20211117 PL - Switzerland TA - Materials (Basel) JT - Materials (Basel, Switzerland) JID - 101555929 PMC - PMC8624380 OTO - NOTNLM OT - alkaline electrolyzed water OT - cement hydration OT - durability OT - fly ash OT - mechanical properties OT - microstructural methods OT - workability COIS- The authors declare no conflict of interest. EDAT- 2021/11/28 06:00 MHDA- 2021/11/28 06:01 PMCR- 2021/11/17 CRDT- 2021/11/27 01:18 PHST- 2021/09/28 00:00 [received] PHST- 2021/11/02 00:00 [revised] PHST- 2021/11/10 00:00 [accepted] PHST- 2021/11/27 01:18 [entrez] PHST- 2021/11/28 06:00 [pubmed] PHST- 2021/11/28 06:01 [medline] PHST- 2021/11/17 00:00 [pmc-release] AID - ma14226956 [pii] AID - materials-14-06956 [pii] AID - 10.3390/ma14226956 [doi] PST - epublish SO - Materials (Basel). 2021 Nov 17;14(22):6956. doi: 10.3390/ma14226956.