PMID- 34938980
OWN - NLM
STAT- PubMed-not-MEDLINE
LR  - 20220925
IS  - 2577-8161 (Electronic)
IS  - 2577-8161 (Linking)
VI  - 3
IP  - 5
DP  - 2021 Sep 24
TI  - Practical implications of perfluoroalkyl substances adsorption on bottle 
      materials: Isotherms.
LID - 10.1002/aws2.1243 [doi]
AB  - To assess the practical implications of various bottle materials used in anion 
      exchange (IX) or granular activated carbon (GAC) isotherm experiments, adsorption 
      of seven per- and polyfluoroalkyl substances (PFAS) onto three common bottle 
      materials (silanized glass, polypropylene, and high-density polyethylene [HDPE]) 
      were screened. Results were similar between bottle materials; therefore, only 
      HDPE was used in a detailed bottle material isotherm study with 11 PFAS. For each 
      PFAS, an HDPE bottle isotherm was generated with equilibrium liquid phase 
      concentrations relevant to drinking water (<2000 ng/L). Percent PFAS recoveries 
      between 90% and 103%, 85% and 114%, and 54% and 108% were determined for 
      perfluoro-2-propoxypropanoic acid (GenX), five perfluoroalkyl carboxylic acids, 
      and five perfluoroalkyl sulfonic acids (PFSA), respectively. These results 
      indicated only the five PFSA adsorbed to the HDPE bottles in a 
      concentration-dependent manner. Furthermore, linear isomer versions of two PFSA 
      exhibited greater adsorption. For each PFSA studied, a linear isotherm was 
      generated and used to develop guidance for conducting future IX and GAC isotherm 
      studies. Specifically, the minimum initial isotherm concentration was established 
      such that a maximum 1% loss would be expected to the HDPE bottles, resulting in 
      required initial concentrations of the five PFSA between 21 and 75 times that of 
      the design isotherm liquid equilibrium concentration.
FAU - Kleiner, Eric J
AU  - Kleiner EJ
AUID- ORCID: 0000-0002-8307-8625
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
FAU - Sanan, Toby
AU  - Sanan T
AUID- ORCID: 0000-0002-0186-2089
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
FAU - Smith, Samantha J
AU  - Smith SJ
AUID- ORCID: 0000-0003-3142-3981
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
FAU - Pressman, Jonathan G
AU  - Pressman JG
AUID- ORCID: 0000-0001-6203-7421
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
FAU - Abulikemu, Gulizhaer
AU  - Abulikemu G
AUID- ORCID: 0000-0001-9614-3505
AD  - Pegasus Technical Services, Inc., Cincinnati, Ohio, USA.
FAU - Crone, Brian C
AU  - Crone BC
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
FAU - Wahman, David G
AU  - Wahman DG
AUID- ORCID: 0000-0002-0167-8468
AD  - United States Environmental Protection Agency, Office of Research and 
      Development, Center for Environmental Solutions and Emergency Response, 
      Cincinnati, Ohio, USA.
LA  - eng
GR  - EPA999999/ImEPA/Intramural EPA/United States
PT  - Journal Article
PL  - United States
TA  - AWWA Water Sci
JT  - AWWA water science
JID - 101743241
PMC - PMC8687106
MID - NIHMS1749646
OTO - NOTNLM
OT  - PFAS
OT  - adsorption
OT  - bottle materials
OT  - drinking water
OT  - isotherm
COIS- CONFLICT OF INTEREST The authors declare no potential conflict of interest.
EDAT- 2021/12/24 06:00
MHDA- 2021/12/24 06:01
PMCR- 2022/09/24
CRDT- 2021/12/23 05:55
PHST- 2021/12/23 05:55 [entrez]
PHST- 2021/12/24 06:00 [pubmed]
PHST- 2021/12/24 06:01 [medline]
PHST- 2022/09/24 00:00 [pmc-release]
AID - 10.1002/aws2.1243 [doi]
PST - ppublish
SO  - AWWA Water Sci. 2021 Sep 24;3(5):10.1002/aws2.1243. doi: 10.1002/aws2.1243.