PMID- 35121261 OWN - NLM STAT- MEDLINE DCOM- 20220222 LR - 20220222 IS - 1090-2414 (Electronic) IS - 0147-6513 (Linking) VI - 232 DP - 2022 Mar 1 TI - Children's exposure to BC and PM pollution, and respiratory tract deposits during commuting trips to school. PG - 113253 LID - S0147-6513(22)00093-8 [pii] LID - 10.1016/j.ecoenv.2022.113253 [doi] AB - Although children have been identified as a vulnerable group highly susceptible to traffic-related air pollution, their exposure during school commutes to traffic-related pollutants and the relevant health impact is rarely studied. In this study, we measured black carbon (BC) and particulate matter (PM: PM(1), PM(2.5), and PM(10)) concentrations that children are exposed to during their multi-modal (walking, private cars, and e-bikes) commuting trips to schools in Xi'an, China. A multi-parameter inhalation rate assessment model was developed in combination with the Multi-Path Particle Dosimetry (MPPD) model to quantify the deposition dose in different parts of children's respiratory system (head, tracheobronchial (TB), pulmonary (PUL)). Results show that walking to school exposed children to the lowest PM(1), PM(2.5), and BC concentrations, whereas riding an e-bike led to significantly elevated exposure to PM(1) and BC than the other two modes. This is due to children's closer proximity to vehicle tail pipe emissions when they bike to school on road or roadside. The PM and BC concentrations showed remarkable increases in comparison to background concentrations during children's school commutes. Urban background (UB) concentration, traffic volume (TV), time of day, and meteorological parameters could influence a child's personal exposure, and the impact of each factor vary across different transportation modes. Particle size of the pollutant affects its deposition site in the respiratory system. Deposition fractions (DFs) and deposition doses in the head region (DF > 50%) were the highest for PM and BC, for which fine particles (BC, PM(1), and PM(2.5)) were then most easily deposited in the PUL region while coarse particles rarely reach PUL. Children inhaled higher doses of polluted air during active commuting (walking) than passive commuting (private cars, e-bikes), due to longer times of exposure coupled with more active breathing. CI - Copyright (c) 2022 The Authors. Published by Elsevier Inc. All rights reserved. FAU - Gao, Jingwen AU - Gao J AD - School of Automobile, Chang'an University, Chang'an Road, Xi'an 710064 Shaanxi, PR China. FAU - Qiu, Zhaowen AU - Qiu Z AD - School of Automobile, Chang'an University, Chang'an Road, Xi'an 710064 Shaanxi, PR China. Electronic address: qzw@chd.edu.cn. FAU - Cheng, Wen AU - Cheng W AD - China National Heavy Duty Truck Group Co., Ltd. (SINOTRUK), Huaao Road, Jinan, 250101 Shandong, PR China. FAU - Gao, H Oliver AU - Gao HO AD - School of Civil and Environmental Engineering, Cornell University 468 Hollister Hall, Ithaca, 14853 NY, USA. LA - eng PT - Journal Article DEP - 20220201 PL - Netherlands TA - Ecotoxicol Environ Saf JT - Ecotoxicology and environmental safety JID - 7805381 RN - 0 (Air Pollutants) RN - 0 (Particulate Matter) RN - 0 (Vehicle Emissions) SB - IM MH - *Air Pollutants/analysis MH - *Air Pollution/analysis MH - Child MH - Environmental Exposure/analysis MH - Environmental Monitoring/methods MH - Humans MH - Lung/chemistry MH - Particle Size MH - Particulate Matter/analysis MH - Schools MH - Transportation MH - Vehicle Emissions/analysis OTO - NOTNLM OT - BC and PM exposure OT - Children OT - Commuting to school OT - Deposition dose EDAT- 2022/02/06 06:00 MHDA- 2022/02/23 06:00 CRDT- 2022/02/05 05:41 PHST- 2021/09/21 00:00 [received] PHST- 2022/01/23 00:00 [revised] PHST- 2022/01/25 00:00 [accepted] PHST- 2022/02/06 06:00 [pubmed] PHST- 2022/02/23 06:00 [medline] PHST- 2022/02/05 05:41 [entrez] AID - S0147-6513(22)00093-8 [pii] AID - 10.1016/j.ecoenv.2022.113253 [doi] PST - ppublish SO - Ecotoxicol Environ Saf. 2022 Mar 1;232:113253. doi: 10.1016/j.ecoenv.2022.113253. Epub 2022 Feb 1.