PMID- 35498576 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20220716 IS - 2046-2069 (Electronic) IS - 2046-2069 (Linking) VI - 10 IP - 17 DP - 2020 Mar 6 TI - Gold nanoparticle-cellulose/PDMS nanocomposite: a flexible dielectric material for harvesting mechanical energy. PG - 10097-10112 LID - 10.1039/c9ra10811d [doi] AB - Cellulose is an abundant natural piezoelectric polymer and is also a renewable resource of significant importance. Here in this work we realize an enhanced piezoelectric response with cellulose in a polydimethylsiloxane (PDMS) matrix by forming a nanocomposite with the incorporation of gold nanoparticles (Au NPs). In the Au NP-cellulose/PDMS nanocomposite an enhancement in the dielectric constant is recorded due to the presence of cellulose alone and a reduction of dielectric loss is found owing to the presence of Au NPs. This opens the possibility of realizing a nanodielectric material from the nanocomposite under current study. This also indicates the significant potential of the nanocomposite towards energy conversion applications. Subsequently, a mechanical energy harvesting device was fabricated using the Au NP-cellulose/PDMS nanocomposite, which is named as a piezoelectric nanogenerator (PNG). The PNG delivered an enhanced open circuit voltage of approximately 6 V, short circuit current of approximately 700 nA and a peak power density of 8.34 mW m(-2) without performing any electrical poling steps. The PNG could charge a 10 muF capacitor to 6.3 V in 677 s and could light two commercial blue light emitting diodes (LEDs) simultaneously. The PNG exhibited a good energy conversion efficiency of 1.8%. A touch sensor application of the PNG is also shown. CI - This journal is (c) The Royal Society of Chemistry. FAU - Pusty, Manojit AU - Pusty M AUID- ORCID: 0000-0003-1015-4057 AD - Discipline of Metallurgy Engineering and Materials Science, Indian Institute of Technology Indore Simrol Indore 453552 India paras.shirage@gmail.com pmshirage@iiti.ac.in +91-787-5222-331. FAU - Shirage, Parasharam M AU - Shirage PM AUID- ORCID: 0000-0003-2884-7548 AD - Discipline of Metallurgy Engineering and Materials Science, Indian Institute of Technology Indore Simrol Indore 453552 India paras.shirage@gmail.com pmshirage@iiti.ac.in +91-787-5222-331. LA - eng PT - Journal Article DEP - 20200310 PL - England TA - RSC Adv JT - RSC advances JID - 101581657 PMC - PMC9050361 COIS- The authors declare no competing financial interests. EDAT- 2020/03/10 00:00 MHDA- 2020/03/10 00:01 PMCR- 2020/03/10 CRDT- 2022/05/02 07:13 PHST- 2019/12/22 00:00 [received] PHST- 2020/02/28 00:00 [accepted] PHST- 2022/05/02 07:13 [entrez] PHST- 2020/03/10 00:00 [pubmed] PHST- 2020/03/10 00:01 [medline] PHST- 2020/03/10 00:00 [pmc-release] AID - c9ra10811d [pii] AID - 10.1039/c9ra10811d [doi] PST - epublish SO - RSC Adv. 2020 Mar 10;10(17):10097-10112. doi: 10.1039/c9ra10811d. eCollection 2020 Mar 6.