PMID- 35653019
OWN - NLM
STAT- MEDLINE
DCOM- 20221013
LR  - 20221013
IS  - 1614-7499 (Electronic)
IS  - 0944-1344 (Linking)
VI  - 29
IP  - 50
DP  - 2022 Oct
TI  - Spatial and seasonal variation and sources of deposition fluxes of polycyclic 
      aromatic hydrocarbons (PAHs) in Shanghai.
PG  - 75258-75270
LID - 10.1007/s11356-022-20348-1 [doi]
AB  - Spatial and temporal variations of polycyclic aromatic hydrocarbons (PAHs) 
      deposition fluxes and sources may significantly facilitate risk evaluation and 
      pollution control of super megacity in China. A study on PAHs of wet and dry 
      deposition in Shanghai was conducted from January to December of 2019. Seventeen 
      sampling sites located in four functional areas were set, including the Baoshan 
      iron and steel industry area (BS), Jinshan petrochemical industry area (JS), city 
      center (CC), and Chongming agricultural area (CM). A total of 15 PAHs were 
      determined by gas chromatography-mass spectrometry (GC-MS, Agilent 7890A/5975C). 
      PAHs atmospheric deposition flux in winter was highest 
      (3.12 +/- 1.98 mug/(m(2).day), mostly attributed to local emissions accumulation 
      under adverse meteorological diffusion conditions, as well as pollutants 
      transport from northern China during heating season. PAHs deposition fluxes in 
      industrial area (BS and JS) were 3.75 +/- 4.08 mug/(m(2).day) and 
      3.18 +/- 3.62 mug/(m(2).day) respectively, which were greater than those in CC and 
      CM, accounting for 1.91 +/- 1.06 mug/(m(2).day) and 1.41 +/- 0.61 mug/(m(2).day) 
      respectively. Proportional composition and isomer ratios of PAHs indicated that 
      the PAHs deposition in winter and spring samples were more homogeneous, whereas 
      those of summer and autumn seemed to be more variable and dispersed. Positive 
      matrix factorization model were employed to identify the potential sources of 
      PAHs in specific functional areas. A dominance of contribution was attributed to 
      coal combustion (46%) at BS, petroleum volatilization (48%) at JS, biomass 
      burning (55%) at CM, and vehicle emission (49%) at CC. This study highlighted 
      that local urbanization and industrialization have a significant contribution to 
      PAHs deposition to specific functional regions in Shanghai.
CI  - (c) 2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, 
      part of Springer Nature.
FAU - Wu, Jian
AU  - Wu J
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China.
FAU - Sha, Chenyan
AU  - Sha C
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China.
FAU - Li, Dayan
AU  - Li D
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China.
FAU - Shen, Cheng
AU  - Shen C
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China.
FAU - Tang, Hao
AU  - Tang H
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China.
FAU - Huang, Shenfa
AU  - Huang S
AD  - Shanghai Academy of Environmental Sciences, Shanghai, 200233, China. 
      saeshuangsf67@163.com.
LA  - eng
GR  - 19ZR1444100/Natural Science Foundation of Shanghai/
PT  - Journal Article
DEP - 20220602
PL  - Germany
TA  - Environ Sci Pollut Res Int
JT  - Environmental science and pollution research international
JID - 9441769
RN  - 0 (Air Pollutants)
RN  - 0 (Coal)
RN  - 0 (Particulate Matter)
RN  - 0 (Petroleum)
RN  - 0 (Polycyclic Aromatic Hydrocarbons)
RN  - 0 (Vehicle Emissions)
RN  - 12597-69-2 (Steel)
RN  - E1UOL152H7 (Iron)
SB  - IM
MH  - *Air Pollutants/analysis
MH  - China
MH  - Coal/analysis
MH  - Environmental Monitoring/methods
MH  - Iron/analysis
MH  - Particulate Matter/analysis
MH  - *Petroleum/analysis
MH  - *Polycyclic Aromatic Hydrocarbons/analysis
MH  - Seasons
MH  - Steel/analysis
MH  - Vehicle Emissions/analysis
OTO - NOTNLM
OT  - PAHs
OT  - Shanghai
OT  - Source identification
OT  - Spatial and temporal distribution
EDAT- 2022/06/03 06:00
MHDA- 2022/10/14 06:00
CRDT- 2022/06/02 11:18
PHST- 2021/11/08 00:00 [received]
PHST- 2022/04/15 00:00 [accepted]
PHST- 2022/06/03 06:00 [pubmed]
PHST- 2022/10/14 06:00 [medline]
PHST- 2022/06/02 11:18 [entrez]
AID - 10.1007/s11356-022-20348-1 [pii]
AID - 10.1007/s11356-022-20348-1 [doi]
PST - ppublish
SO  - Environ Sci Pollut Res Int. 2022 Oct;29(50):75258-75270. doi: 
      10.1007/s11356-022-20348-1. Epub 2022 Jun 2.