PMID- 35805486 OWN - NLM STAT- MEDLINE DCOM- 20220712 LR - 20220824 IS - 1660-4601 (Electronic) IS - 1661-7827 (Print) IS - 1660-4601 (Linking) VI - 19 IP - 13 DP - 2022 Jun 26 TI - Health Risk Assessment of Heavy Metals in Groundwater of Hainan Island Using the Monte Carlo Simulation Coupled with the APCS/MLR Model. LID - 10.3390/ijerph19137827 [doi] LID - 7827 AB - Groundwater is a significant component of water resources, but drinking groundwater with excessive heavy metals (HMs) is harmful to human health. Currently, quantitative source apportionment and probabilistic health risk assessment of HMs in groundwater are relatively limited. In this study, 60 groundwater samples containing seven HMs were collected from Hainan Island and analyzed by the coupled absolute principal component scores/multiple linear regression (APCS/MLR), the health risk assessment (HRA) and the Monte Carlo simulation (MCS) to quantify the pollution sources of HMs and the health risks. The results show that the high-pollution-value areas of HMs are mainly located in the industry-oriented western region, but the pollution level by HMs in the groundwater in the study area is generally low. The main sources of HMs in the groundwater are found to be the mixed sources of agricultural activities and traffic emissions (39.16%), industrial activities (25.57%) and natural sources (35.27%). Although the non-carcinogenic risks for adults and children are negligible, the carcinogenic risks are at a high level. Through analyzing the relationship between HMs, pollution sources, and health risks, natural sources contribute the most to the health risks, and Cr is determined as the priority control HM. This study emphasizes the importance of quantitative evaluation of the HM pollution sources and probabilistic health risk assessment, which provides an essential basis for water pollution prevention and control in Hainan Island. FAU - Shi, Huanhuan AU - Shi H AD - School of Environmental Studies, China University of Geosciences, Wuhan 430078, China. AD - School of Geography and Information Engineering, China University of Geosciences, Wuhan 430078, China. FAU - Zeng, Min AU - Zeng M AD - Wuhan Center of Geological Survey of China Geological Survey, Wuhan 430205, China. FAU - Peng, Hongxia AU - Peng H AD - School of Geography and Information Engineering, China University of Geosciences, Wuhan 430078, China. FAU - Huang, Changsheng AU - Huang C AD - Wuhan Center of Geological Survey of China Geological Survey, Wuhan 430205, China. FAU - Sun, Huimin AU - Sun H AD - School of Geography and Information Engineering, China University of Geosciences, Wuhan 430078, China. FAU - Hou, Qingqin AU - Hou Q AD - School of Geography and Information Engineering, China University of Geosciences, Wuhan 430078, China. FAU - Pi, Pengcheng AU - Pi P AD - School of Geography and Information Engineering, China University of Geosciences, Wuhan 430078, China. LA - eng PT - Journal Article PT - Research Support, Non-U.S. Gov't DEP - 20220626 PL - Switzerland TA - Int J Environ Res Public Health JT - International journal of environmental research and public health JID - 101238455 RN - 0 (Metals, Heavy) RN - 0 (Soil Pollutants) SB - IM MH - Adult MH - Child MH - China MH - Environmental Monitoring MH - *Groundwater MH - Humans MH - Linear Models MH - *Metals, Heavy/analysis MH - Monte Carlo Method MH - Risk Assessment MH - *Soil Pollutants/analysis PMC - PMC9266011 OTO - NOTNLM OT - APCS/MLR model OT - Monte Carlo simulation OT - health risk OT - heavy metals in groundwater OT - source apportionment COIS- The authors declare no conflict of interest. EDAT- 2022/07/10 06:00 MHDA- 2022/07/14 06:00 PMCR- 2022/06/26 CRDT- 2022/07/09 01:07 PHST- 2022/03/31 00:00 [received] PHST- 2022/06/05 00:00 [revised] PHST- 2022/06/06 00:00 [accepted] PHST- 2022/07/09 01:07 [entrez] PHST- 2022/07/10 06:00 [pubmed] PHST- 2022/07/14 06:00 [medline] PHST- 2022/06/26 00:00 [pmc-release] AID - ijerph19137827 [pii] AID - ijerph-19-07827 [pii] AID - 10.3390/ijerph19137827 [doi] PST - epublish SO - Int J Environ Res Public Health. 2022 Jun 26;19(13):7827. doi: 10.3390/ijerph19137827.