PMID- 35890827 OWN - NLM STAT- MEDLINE DCOM- 20220728 LR - 20220731 IS - 1424-8220 (Electronic) IS - 1424-8220 (Linking) VI - 22 IP - 14 DP - 2022 Jul 8 TI - Easy-Scalable Flexible Sensors Made of Carbon Nanotube-Doped Polydimethylsiloxane: Analysis of Manufacturing Conditions and Proof of Concept. LID - 10.3390/s22145147 [doi] LID - 5147 AB - Carbon nanotube (CNT) reinforced polydimethylsiloxane (PDMS) easy-scalable sensors for human motion monitoring are proposed. First, the analysis of the dispersion procedure of nanoparticles into the polymer matrix shows that the ultrasonication (US) technique provides a higher electrical sensitivity in comparison to three-roll milling (3RM) due to the higher homogeneity of the CNT distribution induced by the cavitation forces. Furthermore, the gauge factor (GF) calculated from tensile tests decreases with increasing the CNT content, as the interparticle distance between CNTs is reduced and, thus, the contribution of the tunnelling mechanisms diminishes. Therefore, the optimum conditions were set at 0.4 CNT wt.% dispersed by US procedure, providing a GF of approximately 37 for large strains. The electrical response under cycling load was tested at 2%, 5%, and 10% strain level, indicating a high robustness of the developed sensors. Thus, this strain sensor is in a privileged position with respect to the state-of-the-art, considering all the characteristics that this type of sensor must accomplish: high GF, high flexibility, high reproducibility, easy manufacturing, and friendly operation. Finally, a proof-of-concept of human motion monitoring by placing a sensor for elbow and finger movements is carried out. The electrical resistance was found to increase, as expected, with the bending angle and it is totally recovered after stretching, indicating that there is no prevalent damage and highlighting the huge robustness and applicability of the proposed materials as wearable sensors. FAU - Del Bosque, Antonio AU - Del Bosque A AUID- ORCID: 0000-0002-8301-2159 AD - Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnologia, Universidad Rey Juan Carlos, C/Tulipan s/n, Mostoles, 28933 Madrid, Spain. FAU - Sanchez-Romate, Xoan F AU - Sanchez-Romate XF AUID- ORCID: 0000-0001-9283-4712 AD - Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnologia, Universidad Rey Juan Carlos, C/Tulipan s/n, Mostoles, 28933 Madrid, Spain. FAU - Sanchez, Maria AU - Sanchez M AUID- ORCID: 0000-0003-2823-5103 AD - Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnologia, Universidad Rey Juan Carlos, C/Tulipan s/n, Mostoles, 28933 Madrid, Spain. FAU - Urena, Alejandro AU - Urena A AUID- ORCID: 0000-0002-5049-7954 AD - Materials Science and Engineering Area, Escuela Superior de Ciencias Experimentales y Tecnologia, Universidad Rey Juan Carlos, C/Tulipan s/n, Mostoles, 28933 Madrid, Spain. LA - eng GR - MULTIFUNC-EVs PID2019-107874RB-I00/Agencia Estatal de Investigacion of Spanish Government/ GR - Project ADITIMAT-CM (S2018/NMT-4411)/Comunidad de Madrid Government/ PT - Journal Article DEP - 20220708 PL - Switzerland TA - Sensors (Basel) JT - Sensors (Basel, Switzerland) JID - 101204366 RN - 0 (Dimethylpolysiloxanes) RN - 0 (Nanotubes, Carbon) SB - IM MH - Dimethylpolysiloxanes MH - Humans MH - Motion MH - *Nanotubes, Carbon MH - Reproducibility of Results MH - *Wearable Electronic Devices PMC - PMC9316376 OTO - NOTNLM OT - PDMS OT - carbon nanotubes OT - human motion monitoring OT - stretchable sensors COIS- The authors declare no conflict of interest. EDAT- 2022/07/28 06:00 MHDA- 2022/07/29 06:00 PMCR- 2022/07/08 CRDT- 2022/07/27 01:41 PHST- 2022/06/14 00:00 [received] PHST- 2022/07/01 00:00 [revised] PHST- 2022/07/07 00:00 [accepted] PHST- 2022/07/27 01:41 [entrez] PHST- 2022/07/28 06:00 [pubmed] PHST- 2022/07/29 06:00 [medline] PHST- 2022/07/08 00:00 [pmc-release] AID - s22145147 [pii] AID - sensors-22-05147 [pii] AID - 10.3390/s22145147 [doi] PST - epublish SO - Sensors (Basel). 2022 Jul 8;22(14):5147. doi: 10.3390/s22145147.