PMID- 36502984
OWN - NLM
STAT- PubMed-not-MEDLINE
DCOM- 20230120
LR  - 20230120
IS  - 1879-1026 (Electronic)
IS  - 0048-9697 (Linking)
VI  - 863
DP  - 2023 Mar 10
TI  - Remediation of environmentally persistent organic pollutants (POPs) by 
      persulfates oxidation system (PS): A review.
PG  - 160818
LID - S0048-9697(22)07921-9 [pii]
LID - 10.1016/j.scitotenv.2022.160818 [doi]
AB  - Over the past few years, persistent organic pollutants (POPs) exhibiting high 
      ecotoxicity have been widely detected in the environment. Persulfate-oxidation 
      hybrid system is one of the most widely used novel advanced oxidation techniques 
      and is based on the persulfate generation of SO(4)(-∙) and ∙OH from persulfate to 
      degrade POPs. The overarching aim of this work is to provide a critical review of 
      the variety of methods of peroxide activation (e.g., light activated persulfate, 
      heat-activated persulfate, ultrasound-activated persulfate, 
      electrochemically-activated persulfate, base-activated persulfate, transition 
      metal activated persulfate, as well as Carbon based material activated 
      persulfate). Specifically, through this article we make an attempt to provide the 
      important characteristics and uses of main activated PS methods, as well as the 
      prevailing mechanisms of activated PS to degrade organic pollutants in water. 
      Finally, the advantages and disadvantages of each activation method are analyzed. 
      This work clearly illustrates the benefits of different persulfate activation 
      technologies, and explores persulfate activation in terms of Sustainable 
      Development Goals, technical feasibility, toxicity assessment, and economics to 
      facilitate the large-scale application of persulfate technologies. It also 
      discusses how to choose the most suitable activation method to degrade different 
      types of POPs, filling the research gap in this area and providing better 
      guidance for future research and engineering applications of persulfates.
CI  - Copyright (c) 2022 Elsevier B.V. All rights reserved.
FAU - Liu, Zhibo
AU  - Liu Z
AD  - College of Environmental Science and Engineering, Jilin Normal University, 
      Haifeng Street, Tiexi Dist, Siping 136000, China.
FAU - Ren, Xin
AU  - Ren X
AD  - College of Environmental Science and Engineering, Jilin Normal University, 
      Haifeng Street, Tiexi Dist, Siping 136000, China; Key Laboratory of Environmental 
      Materials and Pollution Control, Education Department of Jilin Province, Siping 
      136000, China.
FAU - Duan, Xiaoyue
AU  - Duan X
AD  - College of Environmental Science and Engineering, Jilin Normal University, 
      Haifeng Street, Tiexi Dist, Siping 136000, China.
FAU - Sarmah, Ajit K
AU  - Sarmah AK
AD  - The Department of Civil & Environmental Engineering, Faculty of Engineering, The 
      University of Auckland, Private Bag 92019, Auckland 1142, New Zealand. Electronic 
      address: a.sarmah@auckland.ac.nz.
FAU - Zhao, Xuesong
AU  - Zhao X
AD  - College of Environmental Science and Engineering, Jilin Normal University, 
      Haifeng Street, Tiexi Dist, Siping 136000, China; Key Laboratory of Environmental 
      Materials and Pollution Control, Education Department of Jilin Province, Siping 
      136000, China. Electronic address: zhaoxuesong008@163.com.
LA  - eng
PT  - Journal Article
PT  - Review
DEP - 20221208
PL  - Netherlands
TA  - Sci Total Environ
JT  - The Science of the total environment
JID - 0330500
SB  - IM
OTO - NOTNLM
OT  - Hydroxyl radicals
OT  - Metal activation
OT  - Peroxide activation
OT  - Persulfate process
OT  - Polymetallic oxides
OT  - Sulfate radicals
COIS- Declaration of competing interest The authors declare that they have no known 
      competing financial interests or personal relationships that could have appeared 
      to influence the work reported in this paper.
EDAT- 2022/12/13 06:00
MHDA- 2022/12/13 06:01
CRDT- 2022/12/12 08:57
PHST- 2022/08/03 00:00 [received]
PHST- 2022/11/17 00:00 [revised]
PHST- 2022/12/06 00:00 [accepted]
PHST- 2022/12/13 06:00 [pubmed]
PHST- 2022/12/13 06:01 [medline]
PHST- 2022/12/12 08:57 [entrez]
AID - S0048-9697(22)07921-9 [pii]
AID - 10.1016/j.scitotenv.2022.160818 [doi]
PST - ppublish
SO  - Sci Total Environ. 2023 Mar 10;863:160818. doi: 10.1016/j.scitotenv.2022.160818. 
      Epub 2022 Dec 8.