PMID- 36816689 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20230224 IS - 2470-1343 (Electronic) IS - 2470-1343 (Linking) VI - 8 IP - 6 DP - 2023 Feb 14 TI - Not All Sizes of Dust can be Removed by Jumping Condensates on Superhydrophobic Surfaces. PG - 5731-5741 LID - 10.1021/acsomega.2c07328 [doi] AB - It is well known that superhydrophobic surfaces (SHSs) possess self-cleaning ability, either by impacting or rolling water droplets or by self-propelled jumping condensate. However, contaminants that are present in the air are various. Is it possible that these contaminants can all be removed from SHSs by jumping condensate? In this study, hydrophilic SiO(2) micro- or nanoparticles with diameters larger than, comparable to, and smaller than the width of the nanogaps of the SHS were first filled in the nanogaps or suspended on the nanostructures with the help of ethanol, and the resulting SHS was exposed to condensing water vapor. Direct observation through microscopy showed that jumping condensation was still obvious on the SHS that were capped or filled with micro- or nanoparticles. Scanning electron microscopy (SEM) imaging demonstrated that following jumping condensation, particles that possessed diameters significantly smaller or larger than the width of the nanogaps were both removed from the SHS. However, most particles possessing diameters comparable to the width of the nanogaps remained on the SHS. This confirms for the first time that not all contaminants or dust can be removed from an SHS by self-propelled jumping condensate. Furthermore, the study also simply demonstrates that vapor condensation occurs within the nanogaps of the SHS. This study is helpful in further understanding the mechanism of the self-cleaning caused by jumping condensate and exploring the initial formation of condensate droplets on the SHS. CI - (c) 2023 The Authors. Published by American Chemical Society. FAU - Li, Kangning AU - Li K AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. AD - Jinhua Polytechnic, Jinhua 321007, China. FAU - Ma, Dandan AU - Ma D AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. FAU - Zhu, Chenxi AU - Zhu C AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. FAU - Yang, Jintao AU - Yang J AUID- ORCID: 0000-0002-3133-1246 AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. FAU - Zhang, Jing AU - Zhang J AUID- ORCID: 0000-0002-0245-7149 AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. FAU - Feng, Jie AU - Feng J AUID- ORCID: 0000-0001-7228-117X AD - College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou 310014, China. LA - eng PT - Journal Article DEP - 20230206 PL - United States TA - ACS Omega JT - ACS omega JID - 101691658 PMC - PMC9933225 COIS- The authors declare no competing financial interest. EDAT- 2023/02/24 06:00 MHDA- 2023/02/24 06:01 PMCR- 2023/02/06 CRDT- 2023/02/23 09:25 PHST- 2022/11/15 00:00 [received] PHST- 2023/01/23 00:00 [accepted] PHST- 2023/02/23 09:25 [entrez] PHST- 2023/02/24 06:00 [pubmed] PHST- 2023/02/24 06:01 [medline] PHST- 2023/02/06 00:00 [pmc-release] AID - 10.1021/acsomega.2c07328 [doi] PST - epublish SO - ACS Omega. 2023 Feb 6;8(6):5731-5741. doi: 10.1021/acsomega.2c07328. eCollection 2023 Feb 14.