PMID- 36947876 OWN - NLM STAT- PubMed-not-MEDLINE DCOM- 20230406 LR - 20230406 IS - 1944-8252 (Electronic) IS - 1944-8244 (Linking) VI - 15 IP - 13 DP - 2023 Apr 5 TI - Quasi-One-Dimensional ZrS(3) Nanoflakes for Broadband and Polarized Photodetection with High Tuning Flexibility. PG - 16999-17008 LID - 10.1021/acsami.3c00273 [doi] AB - Two-dimensional (2D) layered materials with low crystal symmetries have exhibited unique anisotropic physical properties. Here, we report systematic studies on the photoresponse of field effect transistors (FETs) fabricated using quasi-one-dimensional ZrS(3) nanoflakes. The as-fabricated phototransistors exhibit a broadband photocurrent response from ultraviolet to visible regions, where the responsivity and detectivity can be enhanced via additional gate voltages. Furthermore, benefiting from the strong in-plane anisotropy of ZrS(3), we observe a gate-voltage and illumination wavelength-dependent polarized photocurrent response, while its sub-millisecond-time response speed is also polarization-dependent. Our results demonstrate the flexible tunability of photodetectors based on anisotropic layered semiconductors, which substantially broadens the application of low symmetry layered materials in polarization-sensitive optoelectronic devices. FAU - Chen, Feng AU - Chen F AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Liu, Guangjian AU - Liu G AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Xiao, Zhenyang AU - Xiao Z AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Zhou, Hua AU - Zhou H AUID- ORCID: 0000-0003-4146-6862 AD - School of Physics, Shandong University, Shandanan Street 27, 250100 Jinan, P. R. China. FAU - Fei, Linfeng AU - Fei L AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Wan, Siyuan AU - Wan S AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Liao, Xiaxia AU - Liao X AUID- ORCID: 0000-0003-2796-5729 AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Yuan, Jiaren AU - Yuan J AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. FAU - Zhou, Yangbo AU - Zhou Y AUID- ORCID: 0000-0003-4997-7640 AD - School of Physics and Materials Science, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. AD - Jiangxi Engineering Laboratory for Advanced Functional Thin Films and Jiangxi Key Laboratory for Two-Dimensional Materials, Nanchang University, Nanchang, Jiangxi 330031, P. R. China. LA - eng PT - Journal Article DEP - 20230322 PL - United States TA - ACS Appl Mater Interfaces JT - ACS applied materials & interfaces JID - 101504991 SB - IM OTO - NOTNLM OT - 2D materials OT - anisotropic OT - field effect transistor OT - polarized photodetector OT - zirconium trisulfide EDAT- 2023/03/23 06:00 MHDA- 2023/03/23 06:01 CRDT- 2023/03/22 18:32 PHST- 2023/03/23 06:01 [medline] PHST- 2023/03/23 06:00 [pubmed] PHST- 2023/03/22 18:32 [entrez] AID - 10.1021/acsami.3c00273 [doi] PST - ppublish SO - ACS Appl Mater Interfaces. 2023 Apr 5;15(13):16999-17008. doi: 10.1021/acsami.3c00273. Epub 2023 Mar 22.