PMID- 37553052 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20231020 IS - 1879-1026 (Electronic) IS - 0048-9697 (Linking) VI - 902 DP - 2023 Dec 1 TI - Evaluating the generation of microplastics from an unlikely source: The unintentional consequence of the current plastic recycling process. PG - 166090 LID - S0048-9697(23)04715-0 [pii] LID - 10.1016/j.scitotenv.2023.166090 [doi] AB - This study casts light on the potential of microplastic generation during plastic recycling - an unintended consequence of the process. To date, microplastics have been detected in the wastewater and sludge from plastic recycling facilities; however, generation pathways, factors and minimisation strategies are understudied. The purpose of this study is to identify the factors affecting microplastic generation, namely, plastic type and weathering conditions. The size reduction phase, which involved the mechanical shredding of the plastic waste material, was identified to be the predominate source of microplastic generation. Material type was found to significantly affect microplastic generation rates. Focussing on the microplastic particles in the size range of 0.212-1.18 mm, polycarbonate (PC), polyethylene terephthalate (PET), polypropylene (PP), and high-density polyethylene (HDPE) generated 28,600 +/- 3961, 21,093 +/- 2211, 18,987 +/- 752 and 6807 +/- 393 particles/kg of plastic material shredded, respectively. The significant variations between different plastic types were correlated (R(2) = 0.88) to the hardness of the plastic. Environmental weathering was observed to significantly affect microplastic generation rates. Generation rates increased for PC, PET, PP, and HDPE by 185.05 %, 159.80 %, 123.70 % and 121.74 %, respectively, over a six-month environmental exposure period. The results in this study confirm production of large amounts of microplastics from the plastic recycling industry through its operational processes, which may be a significant source for microplastic pollution if measures to reduce their production and removal from wastewater and sludge are not considered. CI - Copyright (c) 2023 The Authors. Published by Elsevier B.V. All rights reserved. FAU - Stapleton, Michael J AU - Stapleton MJ AD - Strategic Water Infrastructure Laboratory, School of Civil, Mining, Environmental and Architectural Engineering, University of Wollongong, Wollongong, NSW 2522, Australia. FAU - Ansari, Ashley J AU - Ansari AJ AD - Strategic Water Infrastructure Laboratory, School of Civil, Mining, Environmental and Architectural Engineering, University of Wollongong, Wollongong, NSW 2522, Australia. FAU - Ahmed, Aziz AU - Ahmed A AD - School of Civil, Mining, Environmental and Architectural Engineering, University of Wollongong, Wollongong, NSW 2522, Australia. FAU - Hai, Faisal I AU - Hai FI AD - Strategic Water Infrastructure Laboratory, School of Civil, Mining, Environmental and Architectural Engineering, University of Wollongong, Wollongong, NSW 2522, Australia. Electronic address: faisal@uow.edu.au. LA - eng PT - Journal Article DEP - 20230806 PL - Netherlands TA - Sci Total Environ JT - The Science of the total environment JID - 0330500 SB - IM OTO - NOTNLM OT - Contamination OT - Mechanical shredding OT - Microplastic pollution OT - Plastic waste OT - Recycling COIS- Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. EDAT- 2023/08/09 01:05 MHDA- 2023/08/09 01:06 CRDT- 2023/08/08 19:11 PHST- 2023/07/06 00:00 [received] PHST- 2023/08/03 00:00 [revised] PHST- 2023/08/04 00:00 [accepted] PHST- 2023/08/09 01:06 [medline] PHST- 2023/08/09 01:05 [pubmed] PHST- 2023/08/08 19:11 [entrez] AID - S0048-9697(23)04715-0 [pii] AID - 10.1016/j.scitotenv.2023.166090 [doi] PST - ppublish SO - Sci Total Environ. 2023 Dec 1;902:166090. doi: 10.1016/j.scitotenv.2023.166090. Epub 2023 Aug 6.