PMID- 37821040 OWN - NLM STAT- MEDLINE DCOM- 20231106 LR - 20231106 IS - 1873-6424 (Electronic) IS - 0269-7491 (Linking) VI - 338 DP - 2023 Dec 1 TI - Size-resolved emission rates of episodic indoor sources and ultrafine particle dynamics. PG - 122680 LID - S0269-7491(23)01682-2 [pii] LID - 10.1016/j.envpol.2023.122680 [doi] AB - Indoor airborne ultrafine particles (UFPs) are mainly originated from occupant activities, such as candle burning and cooking. Elevated exposure to UFPs has been found to increase oxidative stress and cause DNA damage. UFPs originating from indoor sources undergo dynamic aerosol transformation mechanisms. This study investigates the dynamics of UFPs following episodic indoor releases of the six distinct emission sources: 1) candle, 2) gas stove, 3) clothes dryer, 4) tea & toast, 5) broiled fish, and 6) incense. Based on the analytical model of aerosol dynamic processes, this study reports size-resolved source emission rates along with relative contributions of coagulation, deposition, and ventilation to the particle size distribution dynamics. The study findings indicate a significant variation in the geometric mean diameter (GMD) and size-resolved number concentration over time for the sources that emit a substantial amount of UFPs smaller than 10 nm. As the emission progresses, the UFP number concentrations increase in a log-normal distribution, while the GMD shows a tendency to increase over time. The observed result suggests that coagulation can have a considerable impact on UFP number concentration and size, even during the indoor UFP emission. The estimated emission rates of the six indoor sources appear to follow a log-normal distribution while the emission rate ranges from 10(7) min(-1) to 10(12) min(-1). The indoor UFP concentration and size distribution dynamics are substantially affected by the interplay of the three aerosol loss mechanisms that compete with each other, and this impact varies according to the source type and the indoor environmental conditions. Ultimately, using the aerosol transformation mechanisms examined in this study, researchers can refine exposure assessment for epidemiological studies on indoor ultrafine particles. CI - Copyright (c) 2023 Elsevier Ltd. All rights reserved. FAU - Jeong, Su-Gwang AU - Jeong SG AD - Department of Architectural Engineering, Soongsil University, Seoul, 06978, Republic of Korea. FAU - Wallace, Lance AU - Wallace L AD - Wallace Research, Santa Rosa, CA, 95409, USA. FAU - Rim, Donghyun AU - Rim D AD - Department of Architectural Engineering, Pennsylvania State University, University Park, PA, 16802, USA. Electronic address: drim@psu.edu. LA - eng PT - Journal Article DEP - 20231009 PL - England TA - Environ Pollut JT - Environmental pollution (Barking, Essex : 1987) JID - 8804476 RN - 0 (Particulate Matter) RN - 0 (Air Pollutants) RN - 0 (Aerosols) SB - IM MH - Particulate Matter/analysis MH - *Air Pollutants/analysis MH - Particle Size MH - Environmental Monitoring MH - *Air Pollution, Indoor/analysis MH - Aerosols OTO - NOTNLM OT - Coagulation OT - Deposition OT - Indoor air quality OT - Nanoparticles OT - Size distribution OT - Sources strength COIS- Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. EDAT- 2023/10/12 00:43 MHDA- 2023/11/06 06:42 CRDT- 2023/10/11 19:41 PHST- 2023/03/20 00:00 [received] PHST- 2023/08/17 00:00 [revised] PHST- 2023/10/01 00:00 [accepted] PHST- 2023/11/06 06:42 [medline] PHST- 2023/10/12 00:43 [pubmed] PHST- 2023/10/11 19:41 [entrez] AID - S0269-7491(23)01682-2 [pii] AID - 10.1016/j.envpol.2023.122680 [doi] PST - ppublish SO - Environ Pollut. 2023 Dec 1;338:122680. doi: 10.1016/j.envpol.2023.122680. Epub 2023 Oct 9.