PMID- 38051774 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20231226 IS - 1936-086X (Electronic) IS - 1936-0851 (Linking) VI - 17 IP - 24 DP - 2023 Dec 26 TI - Exciton Polaritons in Emergent Two-Dimensional Semiconductors. PG - 24449-24467 LID - 10.1021/acsnano.3c07993 [doi] AB - The "marriage" of light (i.e., photon) and matter (i.e., exciton) in semiconductors leads to the formation of hybrid quasiparticles called exciton polaritons with fascinating quantum phenomena such as Bose-Einstein condensation (BEC) and photon blockade. The research of exciton polaritons has been evolving into an era with emergent two-dimensional (2D) semiconductors and photonic structures for their tremendous potential to break the current limitations of quantum fundamental study and photonic applications. In this Perspective, the basic concepts of 2D excitons, optical resonators, and the strong coupling regime are introduced. The research progress of exciton polaritons is reviewed, and important discoveries (especially the recent ones of 2D exciton polaritons) are highlighted. Subsequently, the emergent 2D exciton polaritons are discussed in detail, ranging from the realization of the strong coupling regime in various photonic systems to the discoveries of attractive phenomena with interesting physics and extensive applications. Moreover, emerging 2D semiconductors, such as 2D perovskites (2DPK) and 2D antiferromagnetic (AFM) semiconductors, are surveyed for the manipulation of exciton polaritons with distinct control degrees of freedom (DOFs). Finally, the outlook on the 2D exciton polaritons and their nonlinear interactions is presented with our initial numerical simulations. This Perspective not only aims to provide an in-depth overview of the latest fundamental findings in 2D exciton polaritons but also attempts to serve as a valuable resource to prospect explorations of quantum optics and topological photonic applications. FAU - Kang, Haifeng AU - Kang H AD - Key Laboratory of Artificial Micro/Nano Structure of Ministry of Education, School of Physics and Technology, Wuhan University, Wuhan, 430072, P. R. China. FAU - Ma, Jingwen AU - Ma J AD - Faculty of Science and Engineering, The University of Hong Kong, Hong Kong, SAR, P. R. China. FAU - Li, Junyu AU - Li J AD - Key Laboratory of Artificial Micro/Nano Structure of Ministry of Education, School of Physics and Technology, Wuhan University, Wuhan, 430072, P. R. China. FAU - Zhang, Xiang AU - Zhang X AD - Faculty of Science and Engineering, The University of Hong Kong, Hong Kong, SAR, P. R. China. AD - Department of Physics, The University of Hong Kong, Hong Kong, SAR, P. R. China. FAU - Liu, Xiaoze AU - Liu X AUID- ORCID: 0000-0002-3586-6408 AD - Key Laboratory of Artificial Micro/Nano Structure of Ministry of Education, School of Physics and Technology, Wuhan University, Wuhan, 430072, P. R. China. AD - Wuhan Institute of Quantum Technology, Wuhan, 430206, P. R. China. AD - Wuhan University Shenzhen Research Institute, Shenzhen, 518057, P. R. China. LA - eng PT - Journal Article PT - Review DEP - 20231205 PL - United States TA - ACS Nano JT - ACS nano JID - 101313589 SB - IM OTO - NOTNLM OT - 2D semiconductors OT - Bose-Einstein condensation OT - exciton polaritons OT - nonlinear interactions OT - strong coupling OT - topological photonics OT - transition metal dichalcogenides (TMDs) OT - valley degree of freedom EDAT- 2023/12/06 03:42 MHDA- 2023/12/06 03:43 CRDT- 2023/12/05 14:03 PHST- 2023/12/06 03:43 [medline] PHST- 2023/12/06 03:42 [pubmed] PHST- 2023/12/05 14:03 [entrez] AID - 10.1021/acsnano.3c07993 [doi] PST - ppublish SO - ACS Nano. 2023 Dec 26;17(24):24449-24467. doi: 10.1021/acsnano.3c07993. Epub 2023 Dec 5.