PMID- 38117279
OWN - NLM
STAT- PubMed-not-MEDLINE
LR  - 20240110
IS  - 1936-086X (Electronic)
IS  - 1936-0851 (Linking)
VI  - 18
IP  - 1
DP  - 2024 Jan 9
TI  - Vertical Phase-Engineering MoS(2) Nanosheet-Enhanced Textiles for Efficient 
      Moisture-Based Energy Generation.
PG  - 492-505
LID - 10.1021/acsnano.3c08132 [doi]
AB  - Flexible moisture-electric generators (MEGs) capture chemical energy from 
      atmospheric moisture for sustainable electricity, gaining attention in wearable 
      electronics. However, challenges persist in the large-scale integration and 
      miniaturization of MEGs for long-term, high-power output. Herein, a vertical 
      heterogeneous phase-engineering MoS(2) nanosheet structure based silk and cotton 
      were rationally designed and successfully applied to construct wearable MEGs for 
      moisture-energy conversion. The prepared METs exhibit  approximately 0.8 V open-circuit 
      voltage,  approximately 0.27 mA/cm(2) current density for >10 h, and >36.12 muW/cm(2) peak 
      output power density, 3 orders higher than current standards. And the large-scale 
      device realizes a current output of 0.145 A. An internal phase gradient between 
      the 2H semiconductor MoS(2) in carbonized silks and 1T metallic MoS(2) in cotton 
      fibers enables a phase-engineering-based heterogeneous electric double layer 
      functioning as an equivalent parallel circuit, leading to enhanced high-power 
      output. Owing to their facile customization for seamless adaptation to the human 
      body, we envision exciting possibilities for these wearable METs as integrated 
      self-power sources, enabling real-time monitoring of physiological parameters in 
      wearable electronics.
FAU - Cao, Yuan-Ming
AU  - Cao YM
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
AD  - College of Biological Science and Medical Engineering, Donghua University, 
      Shanghai 201620, People's Republic of China.
FAU - Su, Yang
AU  - Su Y
AD  - College of Chemistry, Chemical Engineering and Materials Science, Soochow 
      University, Suzhou 215123, People's Republic of China.
FAU - Zheng, Mi
AU  - Zheng M
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
FAU - Luo, Peng
AU  - Luo P
AD  - College of Chemistry, Chemical Engineering and Materials Science, Soochow 
      University, Suzhou 215123, People's Republic of China.
FAU - Xue, Yang-Biao
AU  - Xue YB
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
FAU - Han, Bin-Bin
AU  - Han BB
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
FAU - Zheng, Min
AU  - Zheng M
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
FAU - Wang, Zuoshan
AU  - Wang Z
AUID- ORCID: 0000-0002-3923-0394
AD  - College of Chemistry, Chemical Engineering and Materials Science, Soochow 
      University, Suzhou 215123, People's Republic of China.
FAU - Liao, Liang-Sheng
AU  - Liao LS
AUID- ORCID: 0000-0002-2352-9666
AD  - Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory 
      for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou, 
      Jiangsu 215123, People's Republic of China.
FAU - Zhuo, Ming-Peng
AU  - Zhuo MP
AUID- ORCID: 0000-0003-2399-8160
AD  - College of Textile and Clothing Engineering, Soochow University, Suzhou, Jiangsu 
      215123, People's Republic of China.
AD  - Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory 
      for Carbon-Based Functional Materials & Devices, Soochow University, Suzhou, 
      Jiangsu 215123, People's Republic of China.
LA  - eng
PT  - Journal Article
DEP - 20231220
PL  - United States
TA  - ACS Nano
JT  - ACS nano
JID - 101313589
SB  - IM
OTO - NOTNLM
OT  - energy generation
OT  - moist-electric generators
OT  - molybdenum disulfide
OT  - self-powered sensor
OT  - textile electronics
OT  - two-dimensional materials
OT  - wearable electronics
EDAT- 2023/12/20 12:41
MHDA- 2023/12/20 12:42
CRDT- 2023/12/20 10:43
PHST- 2023/12/20 12:42 [medline]
PHST- 2023/12/20 12:41 [pubmed]
PHST- 2023/12/20 10:43 [entrez]
AID - 10.1021/acsnano.3c08132 [doi]
PST - ppublish
SO  - ACS Nano. 2024 Jan 9;18(1):492-505. doi: 10.1021/acsnano.3c08132. Epub 2023 Dec 
      20.