PMID- 38278878 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20240129 IS - 2045-2322 (Electronic) IS - 2045-2322 (Linking) VI - 14 IP - 1 DP - 2024 Jan 26 TI - The investigation of diesel soot emission using instrument combination of multi-wavelength photoacoustic spectroscopy and scanning mobility particle sizer. PG - 2254 LID - 10.1038/s41598-024-52832-8 [doi] LID - 2254 AB - The parallel measurements of wavelength dependent optical absorption, particle number size distribution have made by a multi wavelength photoacoustic spectrometer (4lambda-PAS) and scanning mobility particle sizer (SMPS) respectively at different modes of a diesel engine using two different types of fuel. The thermal evolution of the emission was also investigated using posterior temperature treatment of emission. The bimodal size distribution of emitted particles at a set reference temperature has been observed regardless of the applied fuel at idle. However, the emitted particulate assembly had lognormal size distribution falls into the accumulation mode at all other defined engine modes and both fuel types. The total number- and volume concentration (TNC and TVC) showed retrograde tendency with the increasing torque and rpm independently of the applied fuel types. The TNC values decreased up to 50% for both fuels with engine operation changes from idle engine mode(em#1) to low engine mode(em#2). With further increase in torque and rpm of engine, the change in TNC is negligible. On the other hand, the TVC remains more or less the same for idle to low engine mode transition and increased more than 60% for high mode (em#3) transition. The Optical Absorption Coefficient (OAC) values measured at the operational wavelengths of the 4lambda-PAS instrument decreased at all wavelengths with increasing rpm and torque. The wavelength dependency quantified by Aerosol Angstrom Exponent (AAE) was applied here for qualitative analysis of the carbonaceous emission and showed decreased values towards the higher engine speed and torque output of the engine. The proposed technique can be used as real-time, precise and accurate measurement of light absorption by DPM aerosols, which opens up novel possibilities for the volatility and thermal evolution investigation of diesel emissions. CI - (c) 2024. The Author(s). FAU - Ajtai, Tibor AU - Ajtai T AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. AD - HUN-REN-SZTE Research Group for Photoacoustic Monitoring of Environmental Processes, Dom ter 9, Szeged, 6720, Hungary. FAU - Utry, Noemi AU - Utry N AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. FAU - Pinter, Mate AU - Pinter M AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. FAU - Rahman, Abdul AU - Rahman A AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. rahman.abdul@szte.hu. FAU - Kurilla, Boldizsar AU - Kurilla B AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. FAU - Sarossy, Gabor AU - Sarossy G AD - MOL Ltd. Duna Refinery, Szazhalombatta, 2440, Hungary. FAU - Deak, Laszlo AU - Deak L AD - MOL Ltd. Duna Refinery, Szazhalombatta, 2440, Hungary. FAU - Baladincz, Jeno AU - Baladincz J AD - MOL Ltd. Duna Refinery, Szazhalombatta, 2440, Hungary. FAU - Raffai, Peter AU - Raffai P AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. FAU - Szabo, Gabor AU - Szabo G AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. FAU - Bozoki, Zoltan AU - Bozoki Z AD - Department of Optics and Quantum Electronics, University of Szeged, 9. Dom Square, Szeged, 6720, Hungary. AD - HUN-REN-SZTE Research Group for Photoacoustic Monitoring of Environmental Processes, Dom ter 9, Szeged, 6720, Hungary. LA - eng PT - Journal Article DEP - 20240126 PL - England TA - Sci Rep JT - Scientific reports JID - 101563288 SB - IM PMC - PMC10817988 COIS- The authors declare no competing interests. EDAT- 2024/01/27 12:42 MHDA- 2024/01/27 12:43 PMCR- 2024/01/26 CRDT- 2024/01/26 23:20 PHST- 2023/12/14 00:00 [received] PHST- 2024/01/24 00:00 [accepted] PHST- 2024/01/27 12:43 [medline] PHST- 2024/01/27 12:42 [pubmed] PHST- 2024/01/26 23:20 [entrez] PHST- 2024/01/26 00:00 [pmc-release] AID - 10.1038/s41598-024-52832-8 [pii] AID - 52832 [pii] AID - 10.1038/s41598-024-52832-8 [doi] PST - epublish SO - Sci Rep. 2024 Jan 26;14(1):2254. doi: 10.1038/s41598-024-52832-8.