PMID- 38360529 OWN - NLM STAT- PubMed-not-MEDLINE LR - 20240229 IS - 1944-8252 (Electronic) IS - 1944-8244 (Linking) VI - 16 IP - 8 DP - 2024 Feb 28 TI - Controlled Preparation of High Quality Bubble-Free and Uniform Conducting Interfaces of Vertical van der Waals Heterostructures of Arrays. PG - 10877-10885 LID - 10.1021/acsami.3c16128 [doi] AB - Sharp and clean interfaces of van der Waals (vdW) heterostructures are highly demanded in two-dimensional (2D) materials-based devices. However, current assembly methods usually cause interfacial bubbles and wrinkles, hindering carrier interlayer transport. The preparation of a large-scale vdW heterostructure with a bubble-free interface is still a challenge. Although many efforts have been made to eliminate bubbles, the evolution processes of the interfacial bubbles are rarely studied. Here, the interface bubble formation and evolution of the transferred 2D materials and their vdW heterostructure are systemically studied by the atomic force microscopy (AFM) technique and high-resolution surface current mapping. A thermal annealing procedure is developed to reduce the number of bubbles and to improve the quality of interfaces. In addition, influences of the interface residues and nanosteps on bubble evolution are also discussed. Further, we develop the polystyrene (PS)-mediated polydimethylsiloxane (PDMS) transfer technique to realize the high-quality transfer of heterostructure arrays. Finally, high-resolution surface current mapping results confirm that we can now produce highly uniform electrical conduction interfaces of heterojunctions. This study provides guidance for assembling high quality interfaces and paves the way for production of bubble-free heterostructure-based electronic devices with high performance and good uniformity. FAU - Chen, Jianwei AU - Chen J AD - State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Province Key Laboratory of Display Material and Technology, School of Electronics and Information Technology, Sun Yat-sen University, Guangzhou 510275, China. FAU - Liu, Liwei AU - Liu L AD - Frontier Institute of Chip and System, Fudan University, Shanghai 200433, China. FAU - Chen, Huanjun AU - Chen H AUID- ORCID: 0000-0003-4699-009X AD - State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Province Key Laboratory of Display Material and Technology, School of Electronics and Information Technology, Sun Yat-sen University, Guangzhou 510275, China. FAU - Xu, Ningsheng AU - Xu N AD - State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Province Key Laboratory of Display Material and Technology, School of Electronics and Information Technology, Sun Yat-sen University, Guangzhou 510275, China. FAU - Deng, Shaozhi AU - Deng S AUID- ORCID: 0000-0003-1830-2026 AD - State Key Laboratory of Optoelectronic Materials and Technologies, Guangdong Province Key Laboratory of Display Material and Technology, School of Electronics and Information Technology, Sun Yat-sen University, Guangzhou 510275, China. LA - eng PT - Journal Article DEP - 20240215 PL - United States TA - ACS Appl Mater Interfaces JT - ACS applied materials & interfaces JID - 101504991 SB - IM OTO - NOTNLM OT - adhesion force OT - array of van der Waals heterostructure OT - atomic force microscopy OT - bubble-free interface OT - surface current mapping EDAT- 2024/02/16 00:43 MHDA- 2024/02/16 00:44 CRDT- 2024/02/15 23:31 PHST- 2024/02/16 00:44 [medline] PHST- 2024/02/16 00:43 [pubmed] PHST- 2024/02/15 23:31 [entrez] AID - 10.1021/acsami.3c16128 [doi] PST - ppublish SO - ACS Appl Mater Interfaces. 2024 Feb 28;16(8):10877-10885. doi: 10.1021/acsami.3c16128. Epub 2024 Feb 15.